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Three-dimensional porous carbon composites containing high sulfur nanoparticle content for high-performance lithium–sulfur batteries
Open accessAbstract
Sulfur is a promising cathode material for lithium–sulfur batteries because of its high theoretical capacity (1,675 mA h g−1); however, its low electrical conductivity and the instability of sulfur-based electrodes limit its practical application. Here we report a facile in situ method for preparing three-dimensional porous graphitic carbon composites containing sulfur nanoparticles (3D S@PGC). With this strategy, the sulfur content of the composites can be tuned to a high level (up to 90 wt%). Because of the high sulfur content, the nanoscale distribution of the sulfur particles, and the covalent bonding between the sulfur and the PGC, the developed 3D S@PGC cathodes exhibit excellent performance, with a high sulfur utilization, high specific capacity (1,382, 1,242 and 1,115 mA h g−1 at 0.5, 1 and 2 C, respectively), long cycling life (small capacity decay of 0.039% per cycle over 1,000 cycles at 2 C) and excellent rate capability at a high charge/discharge current.
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Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Wang, Z., Dong, Y., Li, H., Zhao, Z., Bin Wu, H., Hao, C., Liu, S., Qiu, J., & Lou, X. W. (2014) · Nature Communications · doi:10.1038/ncomms6002 · Cited by 1,059
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Metadata
- Authors
- Li, G., Sun, J., Hou, W., Jiang, S., Huang, Y., & Geng, J.
- Venue
- Nature Communications
- Published
- 2016-02-01
- Volume
- 7
- Issue
- 1
- Pages
- 10601-10601
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2270589204
- Cited by
- 806
- References
- 2
- FWCI
- 60.22
- Type
- journal article
- Language
- en
- Open access
- gold
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- Li, G., Sun, J., Hou, W., Jiang, S., Huang, Y., & Geng, J. (2016). Three-dimensional porous carbon composites containing high sulfur nanoparticle content for high-performance lithium–sulfur batteries. Nature Communications. https://doi.org/10.1038/ncomms10601
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