0.5-keV Soft X-ray attosecond continua
Open accessAbstract
Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element selectivity is a prerequisite, which demands such pulses in the soft X-ray region, above 200 eV, to simultaneously cover several fundamental absorption edges of the constituents of the materials. Here, we experimentally demonstrate the exploitation of a transient phase matching regime to generate carrier envelope controlled soft X-ray supercontinua with pulse energies up to 2.9±0.1 pJ and a flux of (7.3±0.1) × 10 7 photons per second across the entire water window and attosecond pulses with 13 as transform limit. Our results herald attosecond science at the fundamental absorption edges of matter by bridging the gap between ultrafast temporal resolution and element specific probing.
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Isolated attosecond pulses in the water window have recently been demonstrated.
“Recently, isolated attosecond pulses in the water window have been demonstrated [91] (see sections 5.5-5.6).”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [91]
With OPA/OPCPA sources, half-cycle cut-offs in the water window spectral range have been observed, confirming generation of isolated attosecond x-ray pulses in the water window.
“With these OPA/OPCPA sources, half-cycle cut-offs in the water window spectral range have been observed, confirming the generation of isolated attosecond x-ray pulses in the water window [155,156].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [156]
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Mid-Infrared Few-Cycle Pulse Generation and Amplification
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Integrating solids and gases for attosecond pulse generation
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Control of high-order harmonic generation with chirped inhomogeneous fields
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Optical Waveform Synthesis and Its Applications
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Attosecond absorption and reflection spectroscopy of solids
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Spectroscopic Signature of Chemical Bond Dissociation Revealed by Calculated Core-Electron Spectra
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High-order harmonic generation in an x-ray range from laser-induced multivalent ions of noble gas
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Ultrafast magnetic scattering on ferrimagnets enabled by a bright Yb-based soft x-ray source
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Pump−probe experiments at the TEMPO beamline using the low-α operation mode of Synchrotron SOLEIL
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- Authors
- Teichmann, S. M., Silva, F., Cousin, S. L., Hemmer, M., & Biegert, J.
- Affiliations
- Institute of Photonic Sciences (ES)
- Institució Catalana de Recerca i Estudis Avançats (ES)
- Corresponding author
- Biegert, J.
- Venue
- Nature Communications
- Published
- 2016-05-11
- Volume
- 7
- Issue
- 1
- Pages
- 11493-11493
- ISSN
- 2041-1723 (ISSN-L)
- PMC
- PMC4865833
- OpenAlex
- W2337042264
- Cited by
- 265
- References
- 32
- Citations by year
- 2026: 11 · 2025: 20 · 2024: 18 · 2023: 20 · 2022: 33 · 2021: 31 · 2020: 31 · 2019: 47 · 2018: 28 · 2017: 20 · 2016: 6
- FWCI
- 15.92
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Nature Communications (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- arXiv (Cornell University)
- Funders
- Laserlab-Europe (EU-H2020-654148, EU-H2020, 654148)
- European Commission (EU-H2020, 641272, 654148)
- Ministerio de Economía y Competitividad (2015-0522, FIS2014-56774-R, 641272, FIS2014-51478-ERC, SEV2015-0522, 654148, EU-H2020 654148, 2014-2016)
- Horizon 2020 Framework Programme (641272, EU-H2020 654148, 654148)
- Agència de Gestió d'Ajuts Universitaris i de Recerca (SGR 2014, FIS2014-51478-ERC, SGR 2014-2016, SEV-2015-0522)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Keywords
- attosecond pulses, water window, fundamental absorption edge, charge dynamics, ultrafast electron dynamics, attosecond science
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