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Construction of hierarchically porous metal–organic frameworks through linker labilization
Open accessAbstract
A major goal of metal–organic framework (MOF) research is the expansion of pore size and volume. Although many approaches have been attempted to increase the pore size of MOF materials, it is still a challenge to construct MOFs with precisely customized pore apertures for specific applications. Herein, we present a new method, namely linker labilization, to increase the MOF porosity and pore size, giving rise to hierarchical-pore architectures. Microporous MOFs with robust metal nodes and pro-labile linkers were initially synthesized. The mesopores were subsequently created as crystal defects through the splitting of a pro-labile-linker and the removal of the linker fragments by acid treatment. We demonstrate that linker labilization method can create controllable hierarchical porous structures in stable MOFs, which facilitates the diffusion and adsorption process of guest molecules to improve the performances of MOFs in adsorption and catalysis.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Metal–Organic Framework-Based Hierarchically Porous Materials: Synthesis and Applications
Cai, G., Yan, P., Zhang, L., Zhou, H.-C., & Jiang, H.-L. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00243 · Cited by 1,631
Self-citationFrom fundamentals to applications: a toolbox for robust and multifunctional MOF materials
Kirchon, A., Feng, L., Drake, H. F., Joseph, E. A., & Zhou, H.-C. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00688a · Cited by 1,448
Self-citationMetal–Organic Framework-Based Enzyme Biocomposites
Liang, W., Wied, P., Carraro, F., Sumby, C. J., Nidetzky, B., Tsung, C.-K., Falcaro, P., & Doonan, C. J. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c01029 · Cited by 784
Photochemistry and photophysics of MOFs: steps towards MOF-based sensing enhancements
Dolgopolova, E. A., Rice, A. M., Martin, C. R., & Shustova, N. B. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00861a · Cited by 656
Winarta, J., Shan, B., Mcintyre, S. M., Ye, L., Wang, C., Liu, J., & Mu, B. (2020) · Crystal Growth & Design · doi:10.1021/acs.cgd.9b00955 · Cited by 641
Metadata
- Authors
- Yuan, S., Zou, L., Qin, J.-S., Li, J., Huang, L., Feng, L., Wang, X., Bosch, M., Alsalme, A., Cagin, T., & Zhou, H.-C.
- Venue
- Nature Communications
- Published
- 2017-05-25
- Volume
- 8
- Issue
- 1
- Pages
- 15356-15356
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2619486393
- Cited by
- 467
- References
- 1
- FWCI
- 17.86
- Type
- journal article
- Language
- en
- Open access
- gold
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- Yuan, S., Zou, L., Qin, J.-S., Li, J., Huang, L., Feng, L., Wang, X., Bosch, M., Alsalme, A., Cagin, T., & Zhou, H.-C. (2017). Construction of hierarchically porous metal–organic frameworks through linker labilization. Nature Communications. https://doi.org/10.1038/ncomms15356
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