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In situ dynamic observations of perovskite crystallisation and microstructure evolution intermediated from [PbI6]4− cage nanoparticles
Open accessAbstract
Hybrid lead halide perovskites have emerged as high-performance photovoltaic materials with their extraordinary optoelectronic properties. In particular, the remarkable device efficiency is strongly influenced by the perovskite crystallinity and the film morphology. Here, we investigate the perovskites crystallisation kinetics and growth mechanism in real time from liquid precursor continually to the final uniform film. We utilize some advanced in situ characterisation techniques including synchrotron-based grazing incident X-ray diffraction to observe crystal structure and chemical transition of perovskites. The nano-assemble model from perovskite intermediated [PbI 6]4− cage nanoparticles to bulk polycrystals is proposed to understand perovskites formation at a molecular- or nano-level. A crystallisation-depletion mechanism is developed to elucidate the periodic crystallisation and the kinetically trapped morphology at a mesoscopic level. Based on these in situ dynamics studies, the whole process of the perovskites formation and transformation from the molecular to the microstructure over relevant temperature and time scales is successfully demonstrated.
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Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
Impact of microstructure on local carrier lifetime in perovskite solar cells
de Quilettes, D. W., Vorpahl, S. M., Stranks, S. D., Nagaoka, H., Eperon, G. E., Ziffer, M. E., Snaith, H. J., & Ginger, D. S. (2015) · Science · doi:10.1126/science.aaa5333 · Cited by 2,198
Cited by
Scalable fabrication and coating methods for perovskite solar cells and solar modules
Park, N.-G., & Zhu, K. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0176-2 · Cited by 908
Perovskite precursor solution chemistry: from fundamentals to photovoltaic applications
Jung, M., Ji, S.-G., Kim, G., & Seok, S. I. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00656c · Cited by 816
A general approach to high-efficiency perovskite solar cells by any antisolvent
Taylor, A. D., Sun, Q., Goetz, K. P., An, Q., Schramm, T., Hofstetter, Y., Litterst, M., Paulus, F., & Vaynzof, Y. (2021) · Nature Communications · doi:10.1038/s41467-021-22049-8 · Cited by 451
Li, M., Sun, R., Chang, J., Dong, J., Tian, Q., Wang, H., Li, Z., Yang, P., Shi, H., Yang, C., et al. (2023) · Nature Communications · doi:10.1038/s41467-023-36224-6 · Cited by 369
Local Crystal Misorientation Influences Non-radiative Recombination in Halide Perovskites
Jariwala, S., Sun, H., Adhyaksa, G. W. P., Lof, A., Muscarella, L. A., Ehrler, B., Garnett, E. C., & Ginger, D. S. (2019) · Joule · doi:10.1016/j.joule.2019.09.001 · Cited by 273
Metadata
- Authors
- Hu, Q., Zhao, L., Wu, J., Gao, K., Luo, D., Jiang, Y., Zhang, Z., Zhu, C., Schaible, E., Hexemer, A., Wang, C., Liu, Y., Zhang, W., Grätzel, M., Liu, F., Russell, T. P., Zhu, R., & Gong, Q.
- Venue
- Nature Communications
- Published
- 2017-06-21
- Volume
- 8
- Issue
- 1
- Pages
- 15688-15688
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2662873333
- Cited by
- 259
- References
- 2
- FWCI
- 11.30
- Type
- journal article
- Language
- en
- Open access
- gold
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- Hu, Q., Zhao, L., Wu, J., Gao, K., Luo, D., Jiang, Y., Zhang, Z., Zhu, C., Schaible, E., Hexemer, A., Wang, C., Liu, Y., Zhang, W., Grätzel, M., Liu, F., Russell, T. P., Zhu, R., & Gong, Q. (2017). In situ dynamic observations of perovskite crystallisation and microstructure evolution intermediated from [PbI6]4− cage nanoparticles. Nature Communications. https://doi.org/10.1038/ncomms15688
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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