Atomic Auger Doppler effects upon emission of fast photoelectrons
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Studies of photoemission processes induced by hard X-rays including production of energetic electrons have become feasible due to recent substantial improvement of instrumentation. Novel dynamical phenomena have become possible to investigate in this new regime. Here we show a significant change in Auger emission following 1s photoionization of neon, which we attribute to the recoil of the Ne ion induced by the emission of a fast photoelectron. Because of the preferential motion of the ionized Ne atoms along two opposite directions, an Auger Doppler shift is revealed, which manifests itself as a gradual broadening and doubling of the Auger spectral features. This Auger Doppler effect should be a general phenomenon in high-energy photoemission of both isolated atoms and molecules, which will have to be taken into account in studies of other recoil effects such as vibrational or rotational recoil in molecules, and may also have consequences in measurements in solids.
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At high photon energy, the large kinetic energy of the escaping photoelectron induces large translational recoil observed via the atomic Doppler Auger effect.
“At high photon energy, the large kinetic energy of the escaping photoelectron induces large translational recoil observed via the atomic Doppler Auger effect [28]”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [28]
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Roadmap of ultrafast x-ray atomic and molecular physics
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- Authors
- Simon, M., Püttner, R., Marchenko, T., Guillemin, R., Kushawaha, R. K., Journel, L., Goldsztejn, G., Piancastelli, M. N., Ablett, J. M., Rueff, J.-P., & Céolin, D.
- Affiliations
- Centre National de la Recherche Scientifique (FR)
- Freie Universität Berlin (DE)
- Uppsala University (SE)
- Synchrotron SOLEIL (FR)
- Corresponding author
- Piancastelli, Maria Novella
- ORCID
- Venue
- Nature Communications
- Published
- 2014-06-06
- Volume
- 5
- Issue
- 1
- Pages
- 4069-4069
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W1994544220
- Cited by
- 51
- References
- 31
- Citations by year
- 2026: 1 · 2024: 2 · 2023: 2 · 2022: 3 · 2021: 9 · 2020: 4 · 2019: 7 · 2018: 5 · 2017: 4 · 2016: 4 · 2015: 10
- FWCI
- 2.99
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Nature Communications (publishedVersion)
- PubMed (publishedVersion)
- HAL (submittedVersion)
- RePEc: Research Papers in Economics (submittedVersion)
- Funders
- Deutsche Forschungsgemeinschaft (PU 180/6-1)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Materials Science › Surfaces, Coatings and Films › Electron and X-Ray Spectroscopy Techniques
- Keywords
- neon atom, Auger electron spectra, hard X-ray photoemission
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