Cited by 11Atomic and Molecular PhysicsX-ray Spectroscopy and Fluorescence AnalysisLaser-Matter Interactions and Applications

New achievements on relaxation dynamics of atoms and molecules photoexcited in the tender x-ray domain at synchrotron SOLEIL

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Piancastelli, M N, Guillemin, R, Marchenko, T, Journel, L, Travnikova, O, Marin, T, Goldsztejn, G, de Miranda, B Cunha +2 more·2017·Journal of Physics B: Atomic, Molecular and Optical Physics

Abstract

The so-called ‘tender’ x-ray domain, from 2 to 13 keV, has recently become available for atomic and molecular studies at the French synchrotron SOLEIL with state-of-the-art photon and electron energy resolution. We investigated a wealth of new phenomena by means of photoelectron and Auger spectroscopy and electron–ion coincidence techniques. The list includes recoil due to the photoelectron’s momentum, ultrafast nuclear motion on the femto- and sub-femtosecond time scale, double-core-hole studies, electron recapture effects, exotic Auger decay pathways, deep-edge molecular-frame photoelectron angular distribution studies, and core-hole localization/delocalization phenomena for deep-core vacancies. We demonstrate that the newly accessible extended photon energy range does not simply allow studying more systems with deeper core edges, but opens a totally new horizon in what concerns electron and nuclear dynamics of deep-core-excited and core-ionized isolated species.

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  • Because of the short core-hole lifetimes and large kinetic energies of the emitted Auger electrons, just above threshold large post collision interactions (Coulomb interactions between the photoelectron, Auger and the ion) as well as recapture of the photoelectron have been observed.

    “Because of the short core-hole lifetimes and large kinetic energies of the emitted Auger electrons, just above threshold large post collision interactions (Coulomb interactions between the photoelectron, Auger and the ion) as well as recapture of the photoelectron have been observed [23].”

    From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [23]

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Authors
Piancastelli, M. N., Guillemin, R., Marchenko, T., Journel, L., Travnikova, O., Marin, T., Goldsztejn, G., de Miranda, B. C., Ismail, I., & Simon, M.
Affiliations
  • Uppsala University (SE)
  • Centre National de la Recherche Scientifique (FR)
  • Sorbonne Universités
Corresponding author
Simon, M
Venue
Journal of Physics B: Atomic, Molecular and Optical Physics
Published
2017-01-20
Volume
50
Issue
4
Pages
042001
ISSN
  • 0953-4075 (ISSN-L)
  • 1361-6455
OpenAlex
W2574527075
Cited by
11
References
91
Citations by year
2025: 2 · 2023: 2 · 2022: 2 · 2021: 1 · 2018: 4
FWCI
0.54
Type
journal article
Language
en
Open access
Locations
  • Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion)
  • HAL (submittedVersion)
Funders
  • Labex Plas@Par
  • ANR SUMMIT
Topics
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
  • Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
  • Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
Keywords
relaxation dynamics, double-core-hole states, photoelectron angular distributions, core-hole localization, electron-ion coincidence spectroscopy, SOLEIL synchrotron

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