New achievements on relaxation dynamics of atoms and molecules photoexcited in the tender x-ray domain at synchrotron SOLEIL
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The so-called ‘tender’ x-ray domain, from 2 to 13 keV, has recently become available for atomic and molecular studies at the French synchrotron SOLEIL with state-of-the-art photon and electron energy resolution. We investigated a wealth of new phenomena by means of photoelectron and Auger spectroscopy and electron–ion coincidence techniques. The list includes recoil due to the photoelectron’s momentum, ultrafast nuclear motion on the femto- and sub-femtosecond time scale, double-core-hole studies, electron recapture effects, exotic Auger decay pathways, deep-edge molecular-frame photoelectron angular distribution studies, and core-hole localization/delocalization phenomena for deep-core vacancies. We demonstrate that the newly accessible extended photon energy range does not simply allow studying more systems with deeper core edges, but opens a totally new horizon in what concerns electron and nuclear dynamics of deep-core-excited and core-ionized isolated species.
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Because of the short core-hole lifetimes and large kinetic energies of the emitted Auger electrons, just above threshold large post collision interactions (Coulomb interactions between the photoelectron, Auger and the ion) as well as recapture of the photoelectron have been observed.
“Because of the short core-hole lifetimes and large kinetic energies of the emitted Auger electrons, just above threshold large post collision interactions (Coulomb interactions between the photoelectron, Auger and the ion) as well as recapture of the photoelectron have been observed [23].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [23]
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Self-citation
- Authors
- Piancastelli, M. N., Guillemin, R., Marchenko, T., Journel, L., Travnikova, O., Marin, T., Goldsztejn, G., de Miranda, B. C., Ismail, I., & Simon, M.
- Affiliations
- Uppsala University (SE)
- Centre National de la Recherche Scientifique (FR)
- Sorbonne Universités
- Corresponding author
- Simon, M
- ORCID
- Venue
- Journal of Physics B: Atomic, Molecular and Optical Physics
- Publisher
- IOP Publishing
- Published
- 2017-01-20
- Volume
- 50
- Issue
- 4
- Pages
- 042001
- ISSN
- 0953-4075 (ISSN-L)
- 1361-6455
- OpenAlex
- W2574527075
- Cited by
- 11
- References
- 91
- Citations by year
- 2025: 2 · 2023: 2 · 2022: 2 · 2021: 1 · 2018: 4
- FWCI
- 0.54
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion)
- HAL (submittedVersion)
- Funders
- Labex Plas@Par
- ANR SUMMIT
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Keywords
- relaxation dynamics, double-core-hole states, photoelectron angular distributions, core-hole localization, electron-ion coincidence spectroscopy, SOLEIL synchrotron
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
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