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P2-Na0.6[Cr0.6Ti0.4]O2 cation-disordered electrode for high-rate symmetric rechargeable sodium-ion batteries
Open accessAbstract
Most P2-type layered oxides exhibit Na+/vacancy-ordered superstructures because of strong Na+–Na+ interaction in the alkali metal layer and charge ordering in the transition metal layer. These superstructures evidenced by voltage plateaus in the electrochemical curves limit the Na+ ion transport kinetics and cycle performance in rechargeable batteries. Here we show that such Na+/vacancy ordering can be avoided by choosing the transition metal ions with similar ionic radii and different redox potentials, for example, Cr 3+ and Ti 4+. The designed P2-Na 0.6[Cr 0.6 Ti 0.4]O 2 is completely Na+/vacancy-disordered at any sodium content and displays excellent rate capability and long cycle life. A symmetric sodium-ion battery using the same P2-Na 0.6[Cr 0.6 Ti 0.4]O 2 electrode delivers 75% of the initial capacity at 12C rate. Our contribution demonstrates that the approach of preventing Na+/vacancy ordering by breaking charge ordering in the transition metal layer opens a simple way to design disordered electrode materials with high power density and long cycle life.
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Metadata
- Authors
- Wang, Y., Xiao, R., Hu, Y.-S., Avdeev, M., & Chen, L.
- Venue
- Nature Communications
- Published
- 2015-04-24
- Volume
- 6
- Issue
- 1
- Pages
- 6954-6954
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2076766246
- Cited by
- 592
- References
- 37
- FWCI
- 30.63
- Type
- journal article
- Language
- en
- Open access
- gold
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