The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Determining the location and nearest neighbours of aluminium in zeolites with atom probe tomography
Open accessAbstract
Zeolite catalysis is determined by a combination of pore architecture and Brønsted acidity. As Brønsted acid sites are formed by the substitution of AlO 4 for SiO 4 tetrahedra, it is of utmost importance to have information on the number as well as the location and neighbouring sites of framework aluminium. Unfortunately, such detailed information has not yet been obtained, mainly due to the lack of suitable characterization methods. Here we report, using the powerful atomic-scale analysis technique known as atom probe tomography, the quantitative spatial distribution of individual aluminium atoms, including their three-dimensional extent of segregation. Using a nearest-neighbour statistical analysis, we precisely determine the short-range distribution of aluminium over the different T-sites and determine the most probable Al–Al neighbouring distance within parent and steamed ZSM-5 crystals, as well as assess the long-range redistribution of aluminium upon zeolite steaming.
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Citations
Cites
Quantitatively Probing the Al Distribution in Zeolites
Vjunov, A., Fulton, J. L., Huthwelker, T., Pin, S., Mei, D., Schenter, G. K., Govind, N., Camaioni, D. M., Hu, J. Z., & Lercher, J. A. (2014) · Journal of the American Chemical Society · doi:10.1021/ja501361v · Cited by 251
Self-citation
Cited by
Paolucci, C., Parekh, A. A., Khurana, I., Di Iorio, J. R., Li, H., Albarracin Caballero, J. D., Shih, A. J., Anggara, T., Delgass, W. N., Miller, J. T., et al. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b02651 · Cited by 784
Regulation of the Si/Al ratios and Al distributions of zeolites and their impact on properties
Li, J., Gao, M., Yan, W., & Yu, J. (2023) · Chemical Science · doi:10.1039/d2sc06010h · Cited by 404
Engineering Zeolites for Catalytic Cracking to Light Olefins
Blay, V., Louis, B., Miravalles, R., Yokoi, T., Peccatiello, K. A., Clough, M., & Yilmaz, B. (2017) · ACS Catalysis · doi:10.1021/acscatal.7b02011 · Cited by 277
Sequencing of metals in multivariate metal-organic frameworks
Ji, Z., Li, T., & Yaghi, O. M. (2020) · Science · doi:10.1126/science.aaz4304 · Cited by 272
Zeolite (In)Stability under Aqueous or Steaming Conditions
Heard, C. J., Grajciar, L., Uhlík, F., Shamzhy, M., Opanasenko, M., Čejka, J., & Nachtigall, P. (2020) · Advanced Materials · doi:10.1002/adma.202003264 · Cited by 157
Metadata
- Authors
- Perea, D. E., Arslan, I., Liu, J., Ristanović, Z., Kovarik, L., Arey, B. W., Lercher, J. A., Bare, S. R., & Weckhuysen, B. M.
- Venue
- Nature Communications
- Published
- 2015-07-02
- Volume
- 6
- Issue
- 1
- Pages
- 7589-7589
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2267867968
- Cited by
- 188
- References
- 1
- FWCI
- 7.50
- Type
- journal article
- Language
- en
- Open access
- gold
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- Perea, D. E., Arslan, I., Liu, J., Ristanović, Z., Kovarik, L., Arey, B. W., Lercher, J. A., Bare, S. R., & Weckhuysen, B. M. (2015). Determining the location and nearest neighbours of aluminium in zeolites with atom probe tomography. Nature Communications. https://doi.org/10.1038/ncomms8589
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