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Topological crystalline insulator states in Pb1−xSnxSe

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Dziawa, P., Kowalski, B. J., Dybko, K., Buczko, R., Szczerbakow, A., Szot, M., Łusakowska, E., Balasubramanian, T., Wojek, B. M., Berntsen, M. H., Tjernberg, O., Story, T.·2012·Nature Materials

DOI 10.1038/nmat3449

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Abstract

Topological insulators are a class of quantum materials in which time-reversal symmetry, relativistic effects and an inverted band structure result in the occurrence of electronic metallic states on the surfaces of insulating bulk crystals. These helical states exhibit a Dirac-like energy dispersion across the bulk bandgap, and they are topologically protected. Recent theoretical results have suggested the existence of topological crystalline insulators (TCIs), a class of topological insulators in which crystalline symmetry replaces the role of time-reversal symmetry in ensuring topological protection. In this study we show that the narrow-gap semiconductor Pb(1-x)Sn(x)Se is a TCI for x = 0.23. Temperature-dependent angle-resolved photoelectron spectroscopy demonstrates that the material undergoes a temperature-driven topological phase transition from a trivial insulator to a TCI. These experimental findings add a new class to the family of topological insulators, and we anticipate that they will lead to a considerable body of further research as well as detailed studies of topological phase transitions.

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Self-citation
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“Other TCIs wit similar properties but with a more accessible t pological regime are the alloys PbxSn1−xTe [22], or PbxSn1−xSe [23], in which the Ferm level an be modifi d more easily.”
Background
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Authors: Dziawa, P., Kowalski, B. J., Dybko, K., Buczko, R., Szczerbakow, A., Szot, M., Łusakowska, E., Balasubramanian, T., Wojek, B. M., Berntsen, M. H., Tjernberg, O., & Story, T.
Affiliations: Institute of Physics (PL)
Lund University (SE)
KTH Royal Institute of Technology (SE)
Corresponding author: Tjernberg, O.
Story, T.
ORCID: Dziawa, P.
Kowalski, B. J.
Dybko, K.
Buczko, R.
Szczerbakow, A.
Szot, M.
Łusakowska, E.
Balasubramanian, T.
Wojek, B. M.
Berntsen, M. H.
Tjernberg, O.
Story, T.
Venue: Nature Materials
Publisher: Springer Science and Business Media LLC
Published: 2012-09-30
Volume: 11
Issue: 12
Pages: 1023-1027
ISSN: 1476-1122 (ISSN-L)
1476-4660
DOI: 10.1038/nmat3449
OpenAlex: W1997811253
Semantic Scholar: e2378ddb7a491f990b6be147ab709de5256c2e1a
Cited by: 820
References: 32
Citations by year: 2026: 21 · 2025: 50 · 2024: 37 · 2023: 39 · 2022: 53 · 2021: 61 · 2020: 66 · 2019: 72 · 2018: 88 · 2017: 75 · 2016: 67 · 2015: 79 · 2014: 72 · 2013: 33 · 2012: 7
FWCI: 31.61
Type: journal article
Language: en
Open access: green
arxiv.org
Licence: www.springer.com/tdm (tdm)
www.springer.com/tdm (vor)
Locations: Nature Materials (publishedVersion)
PubMed (publishedVersion)
arXiv (Cornell University) (submittedVersion)
Lund University Publications (Lund University) (submittedVersion)
arXiv (Cornell University)
Funders: European Commission
Knut och Alice Wallenbergs Stiftelse
Vetenskapsrådet
European Regional Development Fund
Topics: Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Topological Materials and Phenomena
Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Advanced Condensed Matter Physics
Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
Keywords: topological crystalline insulators, Pb1-xSnxSe, crystal symmetry, topological phase transition, narrow-gap semiconductors, topological protection, surface states, angle-resolved photoemission

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Topological crystalline insulator states in Pb1−xSnxSe

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