The DOI matches its Crossref record; 38 of the 38 references it cites were found in a registry or an index.
Interpreting attoclock measurements of tunnelling times
Abstract
Resolving in time the dynamics of light absorption by atoms and molecules, and the electronic rearrangement this induces, is among the most challenging goals of attosecond spectroscopy. The attoclock is an elegant approach to this problem, which encodes ionization times in the strong-field regime. However, the accurate reconstruction of these times from experimental data presents a formidable theoretical task. Here, we solve this problem by combining analytical theory with ab initio numerical simulations. We apply our theory to numerical attoclock experiments on the hydrogen atom to extract ionization time delays and analyse their nature. Strong-field ionization is often viewed as optical tunnelling through the barrier created by the field and the core potential. We show that, in the hydrogen atom, optical tunnelling is instantaneous. We also show how calibrating the attoclock using the hydrogen atom opens the way to identifying possible delays associated with multielectron dynamics during strong-field ionization. Understanding the physical mechanisms of photon–atom interactions on ultrafast timescales is challenging, but a new theoretical framework enables the interpretation of attoclock experiments measuring tunnelling times in hydrogen.
Overview
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Citations
Cites
Real-time observation of valence electron motion
Goulielmakis, E., Loh, Z.-H., Wirth, A., Santra, R., Rohringer, N., Yakovlev, V. S., Zherebtsov, S., Pfeifer, T., Azzeer, A. M., Kling, M. F., et al. (2010) · Nature · doi:10.1038/nature09212 · Cited by 1,312
Schultze, M., Fieß, M., Karpowicz, N., Gagnon, J., Korbman, M., Hofstetter, M., Neppl, S., Cavalieri, A. L., Komninos, Y., Mercouris, T., et al. (2010) · Science · doi:10.1126/science.1189401 · Cited by 1,121
High harmonic interferometry of multi-electron dynamics in molecules
Smirnova, O., Mairesse, Y., Patchkovskii, S., Dudovich, N., Villeneuve, D., Corkum, P., & Ivanov, M. Y. (2009) · Nature · doi:10.1038/nature08253 · Cited by 1,114
Self-citationTunneling times: a critical review
Hauge, E. H., & Støvneng, J. A. (1989) · Reviews of Modern Physics · doi:10.1103/revmodphys.61.917 · Cited by 1,073
Attosecond Ionization and Tunneling Delay Time Measurements in Helium
Eckle, P., Pfeiffer, A. N., Cirelli, C., Staudte, A., Dörner, R., Muller, H. G., Büttiker, M., & Keller, U. (2008) · Science · doi:10.1126/science.1163439 · Cited by 838
Self-citationBarrier interaction time in tunneling
Landauer, R., & Martin, T. (1994) · Reviews of Modern Physics · doi:10.1103/revmodphys.66.217 · Cited by 768
Probing Single-Photon Ionization on the Attosecond Time Scale
Klünder, K., Dahlström, J. M., Gisselbrecht, M., Fordell, T., Swoboda, M., Guénot, D., Johnsson, P., Caillat, J., Mauritsson, J., Maquet, A., et al. (2011) · Physical Review Letters · doi:10.1103/physrevlett.106.143002 · Cited by 614
Resolving the time when an electron exits a tunnelling barrier
Shafir, D., Soifer, H., Bruner, B. D., Dagan, M., Mairesse, Y., Patchkovskii, S., Ivanov, M. Y., Smirnova, O., & Dudovich, N. (2012) · Nature · doi:10.1038/nature11025 · Cited by 521
Self-citationEckle, P., Smolarski, M., Schlup, P., Biegert, J., Staudte, A., Schöffler, M., Muller, H. G., Dörner, R., & Keller, U. (2008) · Nature Physics · doi:10.1038/nphys982 · Cited by 490
Self-citationStrong-Field Tunneling without Ionization
Nubbemeyer, T., Gorling, K., Sáenz, A., Eichmann, U., & Sandner, W. (2008) · Physical Review Letters · doi:10.1103/physrevlett.101.233001 · Cited by 420
Attoclock reveals natural coordinates of the laser-induced tunnelling current flow in atoms
Pfeiffer, A. N., Cirelli, C., Smolarski, M., Dimitrovski, D., Abu-samha, M., Madsen, L. B., & Keller, U. (2012) · Nature Physics · doi:10.1038/nphys2125 · Cited by 411
Introduction to attosecond delays in photoionization
Dahlström, J. M., L’Huillier, A., & Maquet, A. (2012) · Journal of Physics B: Atomic, Molecular and Optical Physics · doi:10.1088/0953-4075/45/18/183001 · Cited by 365
Ultrafast resolution of tunneling delay time
Landsman, A. S., Weger, M., Maurer, J., Boge, R., Ludwig, A., Heuser, S., Cirelli, C., Gallmann, L., & Keller, U. (2014) · Optica · doi:10.1364/optica.1.000343 · Cited by 241
Nonadiabatic tunneling in circularly polarized laser fields: Physical picture and calculations
Barth, I., & Smirnova, O. (2011) · Physical Review A · doi:10.1103/physreva.84.063415 · Cited by 226
Self-citationTiming the release in sequential double ionization
Pfeiffer, A. N., Cirelli, C., Smolarski, M., Dörner, R., & Keller, U. (2011) · Nature Physics · doi:10.1038/nphys1946 · Cited by 210
Universal Attosecond Response to the Removal of an Electron
Breidbach, J., & Cederbaum, L. S. (2005) · Physical Review Letters · doi:10.1103/physrevlett.94.033901 · Cited by 191
Smirnova, O., Spanner, M., & Ivanov, M. (2008) · Physical Review A · doi:10.1103/physreva.77.033407 · Cited by 174
Self-citationDelay in Atomic Photoionization
Kheifets, A. S., & Ivanov, I. A. (2010) · Physical Review Letters · doi:10.1103/physrevlett.105.233002 · Cited by 165
Self-citationPhoto-electron momentum spectra from minimal volumes: the time-dependent surface flux method
Tao, L., & Scrinzi, A. (2012) · New Journal of Physics · doi:10.1088/1367-2630/14/1/013021 · Cited by 164
Self-citationProbing Nonadiabatic Effects in Strong-Field Tunnel Ionization
Boge, R., Cirelli, C., Landsman, A. S., Heuser, S., Ludwig, A., Mäurer, J., Weger, M., Gallmann, L., & Keller, U. (2013) · Physical Review Letters · doi:10.1103/physrevlett.111.103003 · Cited by 156
Time delay in valence-shell photoionization of noble-gas atoms
Kheifets, A. S. (2013) · Physical Review A · doi:10.1103/physreva.87.063404 · Cited by 145
Self-citationEckle, P. R. (2008) · Repository for Publications and Research Data (ETH Zurich) · doi:10.3929/ethz-a-005760979 · Cited by 141
Shvetsov-Shilovski, N. I., Dimitrovski, D., & Madsen, L. B. (2012) · Physical Review A · doi:10.1103/physreva.85.023428 · Cited by 126
Time-dependent analytical R -matrix approach for strong-field dynamics. I. One-electron systems
Torlina, L., & Smirnova, O. V. (2012) · Physical Review A · doi:10.1103/physreva.86.043408 · Cited by 125
Self-citationHow Accurate Is the Attosecond Streak Camera?
Ivanov, M., & Smirnova, O. V. (2011) · Physical Review Letters · doi:10.1103/physrevlett.107.213605 · Cited by 123
Self-citationTime-resolved photoemission on the attosecond scale: opportunities and challenges
Pazourek, R., Nagele, S., & Burgdörfer, J. (2013) · Faraday Discussions · doi:10.1039/c3fd00004d · Cited by 116
Elliptical Polarization and Probability of Double Ionization
Wang, X., & Eberly, J. H. (2010) · Physical Review Letters · doi:10.1103/physrevlett.105.083001 · Cited by 116
Time delay between photoemission from the 2p and 2s subshells of neon
Moore, L. R., Lysaght, M., Parker, J. S., van der Hart, H. W., & Taylor, K. T. (2011) · Physical Review A · doi:10.1103/physreva.84.061404 · Cited by 114
Time-dependent analytical R -matrix approach for strong-field dynamics. II. Many-electron systems
Torlina, L., Ivanov, M., Walters, Z. B., & Smirnova, O. V. (2012) · Physical Review A · doi:10.1103/physreva.86.043409 · Cited by 100
Self-citationt-SURFF: fully differential two-electron photo-emission spectra
Scrinzi, A. (2012) · New Journal of Physics · doi:10.1088/1367-2630/14/8/085008 · Cited by 99
Self-citationCarette, T., Dahlström, J. M., Argenti, L., & Lindroth, E. (2013) · Physical Review A · doi:10.1103/physreva.87.023420 · Cited by 92
Breakdown of the independent electron approximation in sequential double ionization
Pfeiffer, A. N., Cirelli, C., Smolarski, M. P., Wang, X., Eberly, J. H., Dörner, R., & Keller, U. (2011) · New Journal of Physics · doi:10.1088/1367-2630/13/9/093008 · Cited by 74
Strong-field ionization of He by elliptically polarized light in attoclock configuration
Ivanov, I. A., & Kheifets, A. S. (2014) · Physical Review A · doi:10.1103/physreva.89.021402 · Cited by 68
Self-citationRecent attoclock measurements of strong field ionization
Pfeiffer, A. N., Cirelli, C., Smolarski, M. P., & Keller, U. (2012) · Chemical Physics · doi:10.1016/j.chemphys.2012.02.005 · Cited by 67
How Key Periodic Orbits Drive Recollisions in a Circularly Polarized Laser Field
Kamor, A., Mauger, F., Chandré, C., & Uzer, T. (2013) · Physical Review Letters · doi:10.1103/physrevlett.110.253002 · Cited by 62
Attosecond correlation dynamics during electron tunnelling from molecules
Walters, Z. B., & Smirnova, O. V. (2010) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/43/16/161002 · Cited by 50
Self-citationAttosecond cascades and time delays in one-electron photoionization
Sukiasyan, S., Ishikawa, K. L., & Ivanov, M. (2012) · Physical Review A · doi:10.1103/physreva.86.033423 · Cited by 26
Self-citationAttosecond prints of electrons
Smirnova, O. V. (2010) · Nature · doi:10.1038/466700a · Cited by 16
Self-citation
Cited by
Attosecond correlation dynamics
Ossiander, M., Siegrist, F., Shirvanyan, V., Pazourek, R., Sommer, A., Latka, T., Guggenmos, A., Nagele, S., Feist, J., Burgdörfer, J., et al. (2017) · Nature Physics · doi:10.1038/nphys3941 · Cited by 269
Metadata
- Authors
- Torlina, L., Morales, F., Kaushal, J., Ivanov, I., Kheifets, A., Zielinski, A., Scrinzi, A., Muller, H. G., Sukiasyan, S., Ivanov, M., & Smirnova, O.
- Venue
- Nature Physics
- Published
- 2015-05-25
- Volume
- 11
- Issue
- 6
- Pages
- 503-508
- ISSN
- 1745-2473 (ISSN-L)
- 1745-2481
- OpenAlex
- W2129576383
- Cited by
- 339
- References
- 38
- FWCI
- 18.85
- Type
- journal article
- Language
- en
- Open access
- closed
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.