The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Efficient coupling of photons to a single molecule and the observation of its resonance fluorescence
Open accessAbstract
Single dye molecules at cryogenic temperatures exhibit many spectroscopic phenomena known from the study of free atoms and are thus promising candidates for experiments in fundamental quantum optics. However, the existing techniques for their detection have either sacrificed information on the coherence of the excited state or have been inefficient. Here, we show that these problems can be addressed by focusing the excitation light near to the extinction cross-section of a molecule. Our detection scheme enables us to explore resonance fluorescence over nine orders of magnitude of excitation intensity and to separate its coherent and incoherent parts. In the strong excitation regime, we demonstrate the first direct observation of the Mollow fluorescence triplet from a single solid-state emitter. Under weak excitation, we report the detection of a single molecule with an incident power as faint as 600 aW, paving the way for studying nonlinear effects with only a few photons.
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Cites
Correlation between Photons in two Coherent Beams of Light
BROWN, R. H., & TWISS, R. Q. (1956) · Nature · doi:10.1038/177027a0 · Cited by 2,573
Atom—Photon Interactions: Basic Process and Appilcations
Cohen‐Tannoudji, C., Dupont‐Roc, J., & Grynberg, G. (1998) · doi:10.1002/9783527617197 · Cited by 2,510
Loudon, R. (2000) · doi:10.1093/oso/9780198501770.001.0001 · Cited by 1,890
Resonance Fluorescence from a Coherently Driven Semiconductor Quantum Dot in a Cavity
Muller, A., Flagg, E. B., Bianucci, P., Wang, X. Y., Deppe, D. G., Ma, W., Zhang, J., Salamo, G. J., Xiao, M., & Shih, C. K. (2007) · Physical Review Letters · doi:10.1103/physrevlett.99.187402 · Cited by 360
Cited by
Microwave photonics with superconducting quantum circuits
Gu, X., Kockum, A. F., Miranowicz, A., Liu, Y.-X., & Nori, F. (2017) · Physics Reports · doi:10.1016/j.physrep.2017.10.002 · Cited by 1,307
Atom–light interactions in photonic crystals
Goban, A., Hung, C.-L., Yu, S.-P., Hood, J. D., Muniz, J. A., Lee, J. H., Martin, M. J., McClung, A. C., Choi, K. S., Chang, D. E., et al. (2014) · Nature Communications · doi:10.1038/ncomms4808 · Cited by 462
Resonantly driven coherent oscillations in a solid-state quantum emitter
Flagg, E. B., Muller, A., Robertson, J. W., Founta, S., Deppe, D. G., Xiao, M., Ma, W., Salamo, G. J., & Shih, C. K. (2009) · Nature Physics · doi:10.1038/nphys1184 · Cited by 342
Ates, S., Ulrich, S. M., Reitzenstein, S., Löffler, A., Forchel, A., & Michler, P. (2009) · Physical Review Letters · doi:10.1103/physrevlett.103.167402 · Cited by 265
Quantum interference of tunably indistinguishable photons from remote organic molecules
Lettow, R., Rezus, Y. L. A., Renn, A., Zumofen, G., Ikonen, E., Götzinger, S., & Sandoghdar, V. (2010) · Physical Review Letters · doi:10.1103/physrevlett.104.123605 · Cited by 157
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Metadata
- Authors
- Wrigge, G., Gerhardt, I., Hwang, J., Zumofen, G., & Sandoghdar, V.
- Venue
- Nature Physics
- Published
- 2007-12-16
- Volume
- 4
- Issue
- 1
- Pages
- 60-66
- ISSN
- 1745-2473 (ISSN-L)
- 1745-2481
- OpenAlex
- W2075303310
- Cited by
- 343
- References
- 4
- FWCI
- 13.24
- Type
- journal article
- Language
- en
- Open access
- green
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- Wrigge, G., Gerhardt, I., Hwang, J., Zumofen, G., & Sandoghdar, V. (2008). Efficient coupling of photons to a single molecule and the observation of its resonance fluorescence. Nature Physics. https://doi.org/10.1038/nphys812
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