The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Iced photochemical reduction to synthesize atomically dispersed metals by suppressing nanocrystal growth
Open accessAbstract
Photochemical solution-phase reactions have been widely applied for the syntheses of nanocrystals. In particular, tuning of the nucleation and growth of solids has been a major area of focus. Here we demonstrate a facile approach to generate atomically dispersed platinum via photochemical reduction of frozen chloroplatinic acid solution using ultraviolet light. Using this iced-photochemical reduction, the aggregation of atoms is prevented, and single atoms are successfully stabilized. The platinum atoms are deposited on various substrates, including mesoporous carbon, graphene, carbon nanotubes, titanium dioxide nanoparticles, and zinc oxide nanowires. The atomically dispersed platinum on mesoporous carbon exhibits efficient catalytic activity for the electrochemical hydrogen evolution reaction, with an overpotential of only 65 mV at a current density of 100 mA cm−2 and long-time durability (>10 h), superior to state-of-the-art platinum/carbon. This iced-photochemical reduction may be extended to other single atoms, for example gold and silver, as demonstrated in this study.
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Cites
A fast and robust algorithm for Bader decomposition of charge density
Henkelman, G., Arnaldsson, A., & Jónsson, H. (2006) · Computational Materials Science · doi:10.1016/j.commatsci.2005.04.010 · Cited by 10,723
Platinum single-atom and cluster catalysis of the hydrogen evolution reaction
Cheng, N., Stambula, S., Wang, D., Banis, M. N., Liu, J., Riese, A., Xiao, B., Li, R., Sham, T.-K., Liu, L.-M., et al. (2016) · Nature Communications · doi:10.1038/ncomms13638 · Cited by 2,072
Self-citationUltrafine jagged platinum nanowires enable ultrahigh mass activity for the oxygen reduction reaction
Li, M., Zhao, Z., Cheng, T., Fortunelli, A., Chen, C.-Y., Yu, R., Zhang, Q., Gu, L., Merinov, B. V., Lin, Z., et al. (2016) · Science · doi:10.1126/science.aaf9050 · Cited by 1,605
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Qiu, H. ‐., Ito, Y., Cong, W., Tan, Y., Liu, P., Hirata, A., Fujita, T., Tang, Z., & Chen, M. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201507381 · Cited by 756
Cited by
Large-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst
Zheng, T., Jiang, K., Ta, N., Hu, Y., Zeng, J., Liu, J., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.10.015 · Cited by 887
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Recent advances in the precise control of isolated single-site catalysts by chemical methods
Li, Z., Wang, D., Wu, Y., & Li, Y. (2018) · National Science Review · doi:10.1093/nsr/nwy056 · Cited by 325
Self-citationCheng, Q., Hu, C., Wang, G., Zou, Z., Yang, H., & Dai, L. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b11524 · Cited by 303
Sarma, B. B., Maurer, F., Doronkin, D. E., & Grunwaldt, J.-D. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00495 · Cited by 291
Metadata
- Authors
- Wei, H., Huang, K., Wang, D., Zhang, R., Ge, B., Ma, J., Wen, B., Zhang, S., Li, Q., Lei, M., Zhang, C., Irawan, J., Liu, L.-M., & Wu, H.
- Venue
- Nature Communications
- Published
- 2017-11-14
- Volume
- 8
- Issue
- 1
- Pages
- 1490-1490
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2768069631
- Cited by
- 427
- References
- 5
- FWCI
- 9.18
- Type
- journal article
- Language
- en
- Open access
- gold
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- Wei, H., Huang, K., Wang, D., Zhang, R., Ge, B., Ma, J., Wen, B., Zhang, S., Li, Q., Lei, M., Zhang, C., Irawan, J., Liu, L.-M., & Wu, H. (2017). Iced photochemical reduction to synthesize atomically dispersed metals by suppressing nanocrystal growth. Nature Communications. https://doi.org/10.1038/s41467-017-01521-4
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