The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Cascade anchoring strategy for general mass production of high-loading single-atomic metal-nitrogen catalysts
Open accessAbstract
Although single-atomically dispersed metal-N x on carbon support (M-NC) has great potential in heterogeneous catalysis, the scalable synthesis of such single-atom catalysts (SACs) with high-loading metal-N x is greatly challenging since the loading and single-atomic dispersion have to be balanced at high temperature for forming metal-N x. Herein, we develop a general cascade anchoring strategy for the mass production of a series of M-NC SACs with a metal loading up to 12.1 wt%. Systematic investigation reveals that the chelation of metal ions, physical isolation of chelate complex upon high loading, and the binding with N-species at elevated temperature are essential to achieving high-loading M-NC SACs. As a demonstration, high-loading Fe-NC SAC shows superior electrocatalytic performance for O 2 reduction and Ni-NC SAC exhibits high electrocatalytic activity for CO 2 reduction. The strategy paves a universal way to produce stable M-NC SAC with high-density metal-N x sites for diverse high-performance applications.
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Cites
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Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation
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Self-citationIn situ electrochemical quantification of active sites in Fe–N/C non-precious metal catalysts
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Cited by
Single-Atom Catalysts across the Periodic Table
Kaiser, S. K., Chen, Z., Faust Akl, D., Mitchell, S., & Pérez-Ramírez, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00576 · Cited by 1,367
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
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Yuan, K., Lützenkirchen-Hecht, D., Li, L., Shuai, L., Li, Y., Cao, R., Qiu, M., Zhuang, X., Leung, M. K. H., Chen, Y., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b11852 · Cited by 1,047
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Hu, Q., Gao, K., Wang, X., Zheng, H., Cao, J., Mi, L., Huo, Q., Yang, H., Liu, J., & He, C. (2022) · Nature Communications · doi:10.1038/s41467-022-31660-2 · Cited by 744
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Metadata
- Authors
- Zhao, L., Zhang, Y., Huang, L.-B., Liu, X.-Z., Zhang, Q.-H., He, C., Wu, Z.-Y., Zhang, L.-J., Wu, J., Yang, W., Gu, L., Hu, J.-S., & Wan, L.-J.
- Venue
- Nature Communications
- Published
- 2019-03-20
- Volume
- 10
- Issue
- 1
- Pages
- 1278-1278
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2923015936
- Cited by
- 865
- References
- 10
- FWCI
- 24.27
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zhao, L., Zhang, Y., Huang, L.-B., Liu, X.-Z., Zhang, Q.-H., He, C., Wu, Z.-Y., Zhang, L.-J., Wu, J., Yang, W., Gu, L., Hu, J.-S., & Wan, L.-J. (2019). Cascade anchoring strategy for general mass production of high-loading single-atomic metal-nitrogen catalysts. Nature Communications. https://doi.org/10.1038/s41467-019-09290-y
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