The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Isolated single atom cobalt in Bi3O4Br atomic layers to trigger efficient CO2 photoreduction
Open accessAbstract
The design of efficient and stable photocatalysts for robust CO 2 reduction without sacrifice reagent or extra photosensitizer is still challenging. Herein, a single-atom catalyst of isolated single atom cobalt incorporated into Bi 3 O 4 Br atomic layers is successfully prepared. The cobalt single atoms in the Bi 3 O 4 Br favors the charge transition, carrier separation, CO 2 adsorption and activation. It can lower the CO 2 activation energy barrier through stabilizing the COOH* intermediates and tune the rate-limiting step from the formation of adsorbed intermediate COOH* to be CO* desorption. Taking advantage of cobalt single atoms and two-dimensional ultrathin Bi 3 O 4 Br atomic layers, the optimized catalyst can perform light-driven CO 2 reduction with a selective CO formation rate of 107.1 µmol g−1 h−1, roughly 4 and 32 times higher than that of atomic layer Bi 3 O 4 Br and bulk Bi 3 O 4 Br, respectively.
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Heterogeneous single-atom catalysis
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Self-citationCO2 photo-reduction: insights into CO2 activation and reaction on surfaces of photocatalysts
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Self-citationSingle‐Atom Pt as Co‐Catalyst for Enhanced Photocatalytic H2 Evolution
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Cited by
Single-Atom Catalysts across the Periodic Table
Kaiser, S. K., Chen, Z., Faust Akl, D., Mitchell, S., & Pérez-Ramírez, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00576 · Cited by 1,367
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
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Self-citationFang, S., Rahaman, M., Bharti, J., Reisner, E., Robert, M., Ozin, G. A., & Hu, Y. H. (2023) · Nature Reviews Methods Primers · doi:10.1038/s43586-023-00243-w · Cited by 834
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Single-atom catalysts for photocatalytic energy conversion
Xue, Z.-H., Luan, D., Zhang, H., & (David) Lou, X. W. (2022) · Joule · doi:10.1016/j.joule.2021.12.011 · Cited by 567
Metadata
- Authors
- Di, J., Chen, C., Yang, S.-Z., Chen, S., Duan, M., Xiong, J., Zhu, C., Long, R., Hao, W., Chi, Z., Chen, H., Weng, Y.-X., Xia, J., Song, L., Li, S., Li, H., & Liu, Z.
- Venue
- Nature Communications
- Published
- 2019-06-28
- Volume
- 10
- Issue
- 1
- Pages
- 2840-2840
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2954031782
- Cited by
- 489
- References
- 31
- FWCI
- 12.27
- Type
- journal article
- Language
- en
- Open access
- gold
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- Di, J., Chen, C., Yang, S.-Z., Chen, S., Duan, M., Xiong, J., Zhu, C., Long, R., Hao, W., Chi, Z., Chen, H., Weng, Y.-X., Xia, J., Song, L., Li, S., Li, H., & Liu, Z. (2019). Isolated single atom cobalt in Bi3O4Br atomic layers to trigger efficient CO2 photoreduction. Nature Communications. https://doi.org/10.1038/s41467-019-10392-w
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