The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Strong metal-support interaction promoted scalable production of thermally stable single-atom catalysts
Open accessAbstract
Single-atom catalysts (SACs) have demonstrated superior catalytic performance in numerous heterogeneous reactions. However, producing thermally stable SACs, especially in a simple and scalable way, remains a formidable challenge. Here, we report the synthesis of Ru SACs from commercial RuO 2 powders by physical mixing of sub-micron RuO 2 aggregates with a MgAl 1.2 Fe 0.8 O 4 spinel. Atomically dispersed Ru is confirmed by aberration-corrected scanning transmission electron microscopy and X-ray absorption spectroscopy. Detailed studies reveal that the dispersion process does not arise from a gas atom trapping mechanism, but rather from anti-Ostwald ripening promoted by a strong covalent metal-support interaction. This synthetic strategy is simple and amenable to the large-scale manufacture of thermally stable SACs for industrial applications.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Self-citationCatalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Resolving ruthenium: XPS studies of common ruthenium materials
Morgan, D. J. (2015) · Surface and Interface Analysis · doi:10.1002/sia.5852 · Cited by 1,199
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Cited by
Zhao, Y., Adiyeri Saseendran, D. P., Huang, C., Triana, C. A., Marks, W. R., Chen, H., Zhao, H., & Patzke, G. R. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00515 · Cited by 802
General synthesis of single-atom catalysts with high metal loading using graphene quantum dots
Xia, C., Qiu, Y., Xia, Y., Zhu, P., King, G., Zhang, X., Wu, Z., Kim, J. Y., Cullen, D. A., Zheng, D., et al. (2021) · Nature Chemistry · doi:10.1038/s41557-021-00734-x · Cited by 699
Qian, K., Chen, H., Li, W., Ao, Z., Wu, Y.-N., & Guan, X. (2021) · Environmental Science & Technology · doi:10.1021/acs.est.0c08805 · Cited by 517
Self-citationSingle-Atom (Iron-Based) Catalysts: Synthesis and Applications
Singh, B., Gawande, M. B., Kute, A. D., Varma, R. S., Fornasiero, P., McNeice, P., Jagadeesh, R. V., Beller, M., & Zbořil, R. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00158 · Cited by 373
Supports promote single-atom catalysts toward advanced electrocatalysis
Xu, H., Zhao, Y., Wang, Q., He, G., & Chen, H. (2022) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.214261 · Cited by 363
Metadata
- Authors
- Liu, K., Zhao, X., Ren, G., Yang, T., Ren, Y., Lee, A. F., Su, Y., Pan, X., Zhang, J., Chen, Z., Yang, J., Liu, X., Zhou, T., Xi, W., Luo, J., Zeng, C., Matsumoto, H., Liu, W., Jiang, Q., Wilson, K., Wang, A., Qiao, B., Li, W., & Zhang, T.
- Venue
- Nature Communications
- Published
- 2020-03-09
- Volume
- 11
- Issue
- 1
- Pages
- 1263-1263
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3009222120
- Cited by
- 343
- References
- 4
- FWCI
- 19.20
- Type
- journal article
- Language
- en
- Open access
- gold
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- Liu, K., Zhao, X., Ren, G., Yang, T., Ren, Y., Lee, A. F., Su, Y., Pan, X., Zhang, J., Chen, Z., Yang, J., Liu, X., Zhou, T., Xi, W., Luo, J., Zeng, C., Matsumoto, H., Liu, W., Jiang, Q., . . . Zhang, T. (2020). Strong metal-support interaction promoted scalable production of thermally stable single-atom catalysts. Nature Communications. https://doi.org/10.1038/s41467-020-14984-9
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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