The DOI matches its Crossref record; 56 of the 56 references it cites were found in a registry or an index.
Efficient wettability-controlled electroreduction of CO2 to CO at Au/C interfaces
Open accessAbstract
The electrochemical CO 2 reduction reaction (CO 2 RR) represents a very promising future strategy for synthesizing carbon-containing chemicals in a more sustainable way. In spite of great progress in electrocatalyst design over the last decade, the critical role of wettability-controlled interfacial structures for CO 2 RR remains largely unexplored. Here, we systematically modify the structure of gas-liquid-solid interfaces over a typical Au/C gas diffusion electrode through wettability modification to reveal its contribution to interfacial CO 2 transportation and electroreduction. Based on confocal laser scanning microscopy measurements, the Cassie-Wenzel coexistence state is demonstrated to be the ideal three phase structure for continuous CO 2 supply from gas phase to Au active sites at high current densities. The pivotal role of interfacial structure for the stabilization of the interfacial CO 2 concentration during CO 2 RR is quantitatively analysed through a newly-developed in-situ fluorescence electrochemical spectroscopic method, pinpointing the necessary CO 2 mass transfer conditions for CO 2 RR operation at high current densities.
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Cites
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Self-citationEnhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Liu, M., Pang, Y., Zhang, B., De Luna, P., Voznyy, O., Xu, J., Zheng, X., Dinh, C. T., Fan, F., Cao, C., et al. (2016) · Nature · doi:10.1038/nature19060 · Cited by 2,000
Nature-inspired superwettability systems
Liu, M., Wang, S., & Jiang, L. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2017.36 · Cited by 1,726
Self-citationAqueous CO2 Reduction at Very Low Overpotential on Oxide-Derived Au Nanoparticles
Chen, Y., Li, C. W., & Kanan, M. W. (2012) · Journal of the American Chemical Society · doi:10.1021/ja309317u · Cited by 1,664
Electrocatalytic Conversion of Carbon Dioxide to Methane and Methanol on Transition Metal Surfaces
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Bioinspired Surfaces with Superwettability: New Insight on Theory, Design, and Applications
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Self-citationÁlvarez, A., Bansode, A., Urakawa, A., Bavykina, A. V., Wezendonk, T. A., Makkee, M., Gascon, J., & Kapteijn, F. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00816 · Cited by 1,600
What Should We Make with CO2 and How Can We Make It?
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Ionic Liquid–Mediated Selective Conversion of CO 2 to CO at Low Overpotentials
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Yan, T., Chen, X., Kumari, L., Lin, J., Li, M., Fan, Q., Chi, H., Meyer, T. J., Zhang, S., & Ma, X. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00514 · Cited by 328
Zhang, C., Xu, Z., Han, N., Tian, Y., Kallio, T., Yu, C., & Jiang, L. (2023) · Science Advances · doi:10.1126/sciadv.add6978 · Cited by 230
Self-citationBioinspired Gas Manipulation for Regulating Multiphase Interactions in Electrochemistry
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Metadata
- Authors
- Shi, R., Guo, J., Zhang, X., Waterhouse, G. I. N., Han, Z., Zhao, Y., Shang, L., Zhou, C., Jiang, L., & Zhang, T.
- Venue
- Nature Communications
- Published
- 2020-06-15
- Volume
- 11
- Issue
- 1
- Pages
- 3028-3028
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3034624833
- Cited by
- 531
- References
- 56
- FWCI
- 13.20
- Type
- journal article
- Language
- en
- Open access
- gold
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- Shi, R., Guo, J., Zhang, X., Waterhouse, G. I. N., Han, Z., Zhao, Y., Shang, L., Zhou, C., Jiang, L., & Zhang, T. (2020). Efficient wettability-controlled electroreduction of CO2 to CO at Au/C interfaces. Nature Communications. https://doi.org/10.1038/s41467-020-16847-9
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