The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Tuning reactivity of Fischer–Tropsch synthesis by regulating TiOx overlayer over Ru/TiO2 nanocatalysts
Open accessAbstract
The activity of Fischer–Tropsch synthesis (FTS) on metal-based nanocatalysts can be greatly promoted by the support of reducible oxides, while the role of support remains elusive. Herein, by varying the reduction condition to regulate the TiOx overlayer on Ru nanocatalysts, the reactivity of Ru/TiO 2 nanocatalysts can be differentially modulated. The activity in FTS shows a volcano-like trend with increasing reduction temperature from 200 to 600 °C. Such a variation of activity is characterized to be related to the activation of CO on the TiOx overlayer at Ru/TiO 2 interfaces. Further theoretical calculations suggest that the formation of reduced TiOx occurs facilely on the Ru surface, and it involves in the catalytic mechanism of FTS to facilitate the CO bond cleavage kinetically. This study provides a deep insight on the mechanism of TiOx overlayer in FTS, and offers an effective approach to tuning catalytic reactivity of metal nanocatalysts on reducible oxides.
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Citations
Cites
Strong metal-support interactions. Group 8 noble metals supported on titanium dioxide
Tauster, S. J., Fung, S. C., & Garten, R. L. (1978) · Journal of the American Chemical Society · doi:10.1021/ja00469a029 · Cited by 3,188
Cited by
Li, Y., Zhang, Y., Qian, K., & Huang, W. (2022) · ACS Catalysis · doi:10.1021/acscatal.1c04854 · Cited by 538
Self-citationStructure Sensitivity of Au‐TiO2 Strong Metal–Support Interactions
Zhang, Y., Liu, J., Qian, K., Jia, A., Li, D., Shi, L., Hu, J., Zhu, J., & Huang, W. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202101928 · Cited by 341
Self-citationWang, X., Yang, X., Pei, G., Yang, J., Liu, J., Zhao, F., Jin, F., Jiang, W., Ben, H., & Zhang, L. (2024) · Carbon Energy · doi:10.1002/cey2.391 · Cited by 66
Self-citationIssues and challenges of Fischer–Tropsch synthesis catalysts
Amin, M., Usman, M., Kella, T., Khan, W. U., Khan, I. A., & Hoon Lee, K. (2024) · Frontiers in Chemistry · doi:10.3389/fchem.2024.1462503 · Cited by 52
Metadata
- Authors
- Zhang, Y., Yang, X., Yang, X., Duan, H., Qi, H., Su, Y., Liang, B., Tao, H., Liu, B., Chen, D., Su, X., Huang, Y., & Zhang, T.
- Venue
- Nature Communications
- Published
- 2020-06-24
- Volume
- 11
- Issue
- 1
- Pages
- 3185-3185
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3037713700
- Cited by
- 245
- References
- 1
- FWCI
- 6.28
- Type
- journal article
- Language
- en
- Open access
- gold
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- Zhang, Y., Yang, X., Yang, X., Duan, H., Qi, H., Su, Y., Liang, B., Tao, H., Liu, B., Chen, D., Su, X., Huang, Y., & Zhang, T. (2020). Tuning reactivity of Fischer–Tropsch synthesis by regulating TiOx overlayer over Ru/TiO2 nanocatalysts. Nature Communications. https://doi.org/10.1038/s41467-020-17044-4
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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