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Heterophase fcc-2H-fcc gold nanorods
Open accessAbstract
The crystal phase-based heterostructures of noble metal nanomaterials are of great research interest for various applications, such as plasmonics and catalysis. However, the synthesis of unusual crystal phases of noble metals still remains a great challenge, making the construction of heterophase noble metal nanostructures difficult. Here, we report a one-pot wet-chemical synthesis of well-defined heterophase fcc-2H-fcc gold nanorods (fcc: face-centred cubic; 2H: hexagonal close-packed with stacking sequence of “AB”) at mild conditions. Single particle-level experiments and theoretical investigations reveal that the heterophase gold nanorods demonstrate a distinct optical property compared to that of the conventional fcc gold nanorods. Moreover, the heterophase gold nanorods possess superior electrocatalytic activity for the carbon dioxide reduction reaction over their fcc counterparts under ambient conditions. First-principles calculations suggest that the boosted catalytic performance stems from the energetically favourable adsorption of reaction intermediates, endowed by the unique heterophase characteristic of gold nanorods.
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Highly Crystalline Multimetallic Nanoframes with Three-Dimensional Electrocatalytic Surfaces
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Ultrafine jagged platinum nanowires enable ultrahigh mass activity for the oxygen reduction reaction
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Self-citationSelective increase in CO 2 electroreduction activity at grain-boundary surface terminations
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Self-citationFemtosecond laser reshaping yields gold nanorods with ultranarrow surface plasmon resonances
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Self-citationLi, L., Liu, C., Liu, S., Wang, J., Han, J., Chan, T.-S., Li, Y., Hu, Z., Shao, Q., Zhang, Q., et al. (2022) · ACS Nano · doi:10.1021/acsnano.2c05776 · Cited by 104
Self-citationToward a Quantitative Understanding of Crystal-Phase Engineering of Ru Nanocrystals
Lin, J.-T., Liu, Y.-H., Tsao, C.-Y., Wu, C.-Y., Hsieh, C.-J., Chen, M.-Z., Chang, C.-W., Hsiao, Y.-C., Chen, H.-L., & Yang, T.-H. (2023) · Chemistry of Materials · doi:10.1021/acs.chemmater.3c00326 · Cited by 15
Metadata
- Authors
- Fan, Z., Bosman, M., Huang, Z., Chen, Y., Ling, C., Wu, L., Akimov, Y. A., Laskowski, R., Chen, B., Ercius, P., Zhang, J., Qi, X., Goh, M. H., Ge, Y., Zhang, Z., Niu, W., Wang, J., Zheng, H., & Zhang, H.
- Venue
- Nature Communications
- Published
- 2020-07-03
- Volume
- 11
- Issue
- 1
- Pages
- 3293-3293
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3038326856
- Cited by
- 161
- References
- 10
- FWCI
- 14.22
- Type
- journal article
- Language
- en
- Open access
- gold
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- Fan, Z., Bosman, M., Huang, Z., Chen, Y., Ling, C., Wu, L., Akimov, Y. A., Laskowski, R., Chen, B., Ercius, P., Zhang, J., Qi, X., Goh, M. H., Ge, Y., Zhang, Z., Niu, W., Wang, J., Zheng, H., & Zhang, H. (2020). Heterophase fcc-2H-fcc gold nanorods. Nature Communications. https://doi.org/10.1038/s41467-020-17068-w
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