The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Thermal runaway of Lithium-ion batteries employing LiN(SO2F)2-based concentrated electrolytes
Open accessAbstract
Concentrated electrolytes usually demonstrate good electrochemical performance and thermal stability, and are also supposed to be promising when it comes to improving the safety of lithium-ion batteries due to their low flammability. Here, we show that LiN(SO 2 F)2-based concentrated electrolytes are incapable of solving the safety issues of lithium-ion batteries. To illustrate, a mechanism based on battery material and characterizations reveals that the tremendous heat in lithium-ion batteries is released due to the reaction between the lithiated graphite and LiN(SO 2 F)2 triggered thermal runaway of batteries, even if the concentrated electrolyte is non-flammable or low-flammable. Generally, the flammability of an electrolyte represents its behaviors when oxidized by oxygen, while it is the electrolyte reduction that triggers the chain of exothermic reactions in a battery. Thus, this study lights the way to a deeper understanding of the thermal runaway mechanism in batteries as well as the design philosophy of electrolytes for safer lithium-ion batteries.
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Citations
Cites
A review on the key issues of the lithium ion battery degradation among the whole life cycle
Han, X., Lu, L., Zheng, Y., Feng, X., Li, Z., Li, J., & Ouyang, M. (2019) · eTransportation · doi:10.1016/j.etran.2019.100005 · Cited by 1,745
Self-citationLithium-ion battery fast charging: A review
Tomaszewska, A., Chu, Z., Feng, X., O'Kane, S., Liu, X., Chen, J., Ji, C., Endler, E., Li, R., Liu, L., et al. (2019) · eTransportation · doi:10.1016/j.etran.2019.100011 · Cited by 1,592
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Cited by
A Review of Solid Electrolyte Interphase (SEI) and Dendrite Formation in Lithium Batteries
Li, B., Chao, Y., Li, M., Xiao, Y., Li, R., Yang, K., Cui, X., Xu, G., Li, L., Yang, C., et al. (2023) · Electrochemical Energy Reviews · doi:10.1007/s41918-022-00147-5 · Cited by 406
Geometry-influenced cooling performance of lithium-ion battery
Dubey, D., Mishra, A., Ghosh, S., Reddy, M. V., & Pandey, R. (2023) · Applied Thermal Engineering · doi:10.1016/j.applthermaleng.2023.120723 · Cited by 25
Metadata
- Authors
- Hou, J., Lu, L., Wang, L., Ohma, A., Ren, D., Feng, X., Li, Y., Li, Y., Ootani, I., Han, X., Ren, W., He, X., Nitta, Y., & Ouyang, M.
- Venue
- Nature Communications
- Published
- 2020-10-09
- Volume
- 11
- Issue
- 1
- Pages
- 5100-5100
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3092189325
- Cited by
- 326
- References
- 2
- FWCI
- 10.97
- Type
- journal article
- Language
- en
- Open access
- gold
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- Hou, J., Lu, L., Wang, L., Ohma, A., Ren, D., Feng, X., Li, Y., Li, Y., Ootani, I., Han, X., Ren, W., He, X., Nitta, Y., & Ouyang, M. (2020). Thermal runaway of Lithium-ion batteries employing LiN(SO2F)2-based concentrated electrolytes. Nature Communications. https://doi.org/10.1038/s41467-020-18868-w
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