The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Skin-like mechanoresponsive self-healing ionic elastomer from supramolecular zwitterionic network
Open accessAbstract
Stretchable ionic skins are intriguing in mimicking the versatile sensations of natural skins. However, for their applications in advanced electronics, good elastic recovery, self-healing, and more importantly, skin-like nonlinear mechanoresponse (strain-stiffening) are essential but can be rarely met in one material. Here we demonstrate a robust proton-conductive ionic skin design via introducing an entropy-driven supramolecular zwitterionic reorganizable network to the hydrogen-bonded polycarboxylic acid network. The design allows two dynamic networks with distinct interacting strength to sequentially debond with stretch, and the conflict among elasticity, self-healing, and strain-stiffening can be thus defeated. The representative polyacrylic acid/betaine elastomer exhibits high stretchability (1600% elongation), immense strain-stiffening (24-fold modulus enhancement), ~100% self-healing, excellent elasticity (97.9 ± 1.1% recovery ratio, <14% hysteresis), high transparency (99.7 ± 0.1%), moisture-preserving, anti-freezing (elastic at −40 °C), water reprocessibility, as well as easy-to-peel adhesion. The combined advantages make the present ionic elastomer very promising in wearable iontronic sensors for human-machine interfacing.
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Cites
Kang, J., Tok, J. B.-H., & Bao, Z. (2019) · Nature Electronics · doi:10.1038/s41928-019-0235-0 · Cited by 706
Wang, M., Luo, Y., Wang, T., Wan, C., Pan, L., Pan, S., He, K., Neo, A., & Chen, X. (2021) · Advanced Materials · doi:10.1002/adma.202003014 · Cited by 451
Highly stretchable and transparent ionic conducting elastomers
Shi, L., Zhu, T., Gao, G., Zhang, X., Wei, W., Liu, W., & Ding, S. (2018) · Nature Communications · doi:10.1038/s41467-018-05165-w · Cited by 337
Cited by
Fu, Q., Hao, S., Meng, L., Xu, F., & Yang, J. (2021) · ACS Nano · doi:10.1021/acsnano.1c08193 · Cited by 346
Chen, J., Gao, Y., Shi, L., Yu, W., Sun, Z., Zhou, Y., Liu, S., Mao, H., Zhang, D., Lu, T., et al. (2022) · Nature Communications · doi:10.1038/s41467-022-32517-4 · Cited by 325
Conductive polymer based hydrogels and their application in wearable sensors: a review
Liu, D., Huyan, C., Wang, Z., Guo, Z., Zhang, X., Torun, H., Mulvihill, D., Xu, B. B., & Chen, F. (2023) · Materials Horizons · doi:10.1039/d3mh00056g · Cited by 282
Xiang, H., Li, X., Wu, B., Sun, S., & Wu, P. (2023) · Advanced Materials · doi:10.1002/adma.202209581 · Cited by 268
Self-citationHumidity Sensing of Stretchable and Transparent Hydrogel Films for Wireless Respiration Monitoring
Liang, Y., Ding, Q., Wang, H., Wu, Z., Li, J., Li, Z., Tao, K., Gui, X., & Wu, J. (2022) · Nano-Micro Letters · doi:10.1007/s40820-022-00934-1 · Cited by 162
Metadata
- Authors
- Zhang, W., Wu, B., Sun, S., & Wu, P.
- Venue
- Nature Communications
- Published
- 2021-07-02
- Volume
- 12
- Issue
- 1
- Pages
- 4082-4082
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W3177384764
- Cited by
- 535
- References
- 3
- FWCI
- 25.27
- Type
- journal article
- Language
- en
- Open access
- gold
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