Integrated halide perovskite photoelectrochemical cells with solar-driven water-splitting efficiency of 20.8%
Open accessAbstract
Achieving high solar-to-hydrogen (STH) efficiency concomitant with long-term durability using low-cost, scalable photo-absorbers is a long-standing challenge. Here we report the design and fabrication of a conductive adhesive-barrier (CAB) that translates >99% of photoelectric power to chemical reactions. The CAB enables halide perovskite-based photoelectrochemical cells with two different architectures that exhibit record STH efficiencies. The first, a co-planar photocathode-photoanode architecture, achieved an STH efficiency of 13.4% and 16.3 h to t 60, solely limited by the hygroscopic hole transport layer in the n-i-p device. The second was formed using a monolithic stacked silicon-perovskite tandem, with a peak STH efficiency of 20.8% and 102 h of continuous operation before t 60 under AM 1.5G illumination. These advances will lead to efficient, durable, and low-cost solar-driven water-splitting technology with multifunctional barriers.
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The high efficiency of a perovskite solar cell (PSC) is associated with a high absorption coefficient, direct bandgap transition, low effective mass, long diffusion length, and relatively high carrier mobility of free electrons and holes.
“The high efficiency of a perovskite solar cell (PSC) is associated with a high absorption coefficient, direct bandgap transition, low effective mass, long diffusion length, and relatively high carrier mobility of free electrons and holes.[162,163]”
From Advances in Blue Energy Fuels: Harvesting Energy from Ocean for Self‐Powered Electrolysis (2025) · cites this paper as [163]
The Introduction links high perovskite solar-cell efficiency to large absorption coefficients and long diffusion lengths, and mentions tunable bandgaps and charge-carrier lifetimes. It does not establish a direct bandgap transition, low effective mass, or relatively high mobility of free electrons and holes as contributors to that efficiency. Page numbers are not available in our copy. (LLM, conf=0.88)
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- Authors
- Fehr, A. M. K., Agrawal, A., Mandani, F., Conrad, C. L., Jiang, Q., Park, S. Y., Alley, O., Li, B., Sidhik, S., Metcalf, I., Botello, C., Young, J. L., Even, J., Blancon, J. C., Deutsch, T. G., Zhu, K., Albrecht, S., Toma, F. M., Wong, M., & Mohite, A. D.
- Affiliations
- Rice University (US)
- National Laboratory of the Rockies (US)
- Lawrence Berkeley National Laboratory (US)
- Helmholtz-Zentrum Berlin für Materialien und Energie (DE)
- Centre National de la Recherche Scientifique (FR)
- Corresponding author
- Wong, Michael
- Mohite, Aditya D.
- ORCID
- Venue
- Nature Communications
- Published
- 2023-06-26
- Volume
- 14
- Issue
- 1
- Pages
- 3797-3797
- ISSN
- 2041-1723 (ISSN-L)
- PMC
- PMC10293190
- OpenAlex
- W4382020723
- Cited by
- 177
- References
- 47
- Citations by year
- 2026: 54 · 2025: 59 · 2024: 54 · 2023: 10
- FWCI
- 8.46
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- Nature Communications (publishedVersion, cc-by)
- PubMed Central (publishedVersion, cc-by)
- PubMed (publishedVersion)
- HAL (submittedVersion, cc-by)
- eScholarship (California Digital Library) (submittedVersion, cc-by)
- RePEc: Research Papers in Economics (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- HZB Repository (Helmholtz-Zentrum Berlin für Materialien und Energie GmbH (HZB)) (submittedVersion, other-oa)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Funders
- DOE | Office of Energy Efficiency and Renewable Energy (DE-EE0008843)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Perovskite Materials and Applications
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › TiO2 Photocatalysis and Solar Cells
- Keywords
- solar water splitting, solar-to-hydrogen efficiency, device durability
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