The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Tunable CO2 electroreduction to ethanol and ethylene with controllable interfacial wettability
Open accessAbstract
The mechanism of how interfacial wettability impacts the CO 2 electroreduction pathways to ethylene and ethanol remains unclear. This paper describes the design and realization of controllable equilibrium of kinetic-controlled *CO and *H via modifying alkanethiols with different alkyl chain lengths to reveal its contribution to ethylene and ethanol pathways. Characterization and simulation reveal that the mass transport of CO 2 and H 2 O is related with interfacial wettability, which may result in the variation of kinetic-controlled *CO and *H ratio, which affects ethylene and ethanol pathways. Through modulating the hydrophilic interface to superhydrophobic interface, the reaction limitation shifts from insufficient supply of kinetic-controlled *CO to that of *H. The ethanol to ethylene ratio can be continuously tailored in a wide range from 0.9 to 1.92, with remarkable Faradaic efficiencies toward ethanol and multi-carbon (C 2+) products up to 53.7% and 86.1%, respectively. A C 2+ Faradaic efficiency of 80.3% can be achieved with a high C 2+ partial current density of 321 mA cm−2, which is among the highest selectivity at such current densities.
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Cites
What would it take for renewably powered electrosynthesis to displace petrochemical processes?
De Luna, P., Hahn, C., Higgins, D., Jaffer, S. A., Jaramillo, T. F., & Sargent, E. H. (2019) · Science · doi:10.1126/science.aav3506 · Cited by 3,052
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
CO 2 electrolysis to multicarbon products at activities greater than 1 A cm −2
García de Arquer, F. P., Dinh, C.-T., Ozden, A., Wicks, J., McCallum, C., Kirmani, A. R., Nam, D.-H., Gabardo, C., Seifitokaldani, A., Wang, X., et al. (2020) · Science · doi:10.1126/science.aay4217 · Cited by 1,517
De Luna, P., Quintero-Bermudez, R., Dinh, C.-T., Ross, M. B., Bushuyev, O. S., Todorović, P., Regier, T., Kelley, S. O., Yang, P., & Sargent, E. H. (2018) · Nature Catalysis · doi:10.1038/s41929-017-0018-9 · Cited by 1,046
Goodpaster, J. D., Bell, A. T., & Head-Gordon, M. (2016) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.6b00358 · Cited by 702
Mechanistic Insights for Low-Overpotential Electroreduction of CO2 to CO on Copper Nanowires
Cao, L., Raciti, D., Li, C., Livi, K. J. T., Rottmann, P. F., Hemker, K. J., Mueller, T., & Wang, C. (2017) · ACS Catalysis · doi:10.1021/acscatal.7b03107 · Cited by 122
Cited by
Jiang, M., Wang, H., Zhu, M., Luo, X., He, Y., Wang, M., Wu, C., Zhang, L., Li, X., Liao, X., et al. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00857f · Cited by 299
Self-citationWang, Y., Zhang, J., Zhao, J., Wei, Y., Chen, S., Zhao, H., Su, Y., Ding, S., & Xiao, C. (2024) · ACS Catalysis · doi:10.1021/acscatal.3c05880 · Cited by 269
Electrocatalytic CO2 hydrogenation to C2+ alcohols catalysed by Pr–Cu oxide heterointerfaces
Liu, J., Li, P., Jia, S., Wang, Y., Jing, L., Liu, Z., Zhang, J., Qian, Q., Kang, X., Sun, X., et al. (2025) · Nature Synthesis · doi:10.1038/s44160-025-00752-4 · Cited by 96
Metadata
- Authors
- Lin, Y., Wang, T., Zhang, L., Zhang, G., Li, L., Chang, Q., Pang, Z., Gao, H., Huang, K., Zhang, P., Zhao, Z.-J., Pei, C., & Gong, J.
- Venue
- Nature Communications
- Published
- 2023-06-16
- Volume
- 14
- Issue
- 1
- Pages
- 3575-3575
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W4380878375
- Cited by
- 275
- References
- 6
- FWCI
- 12.87
- Type
- journal article
- Language
- en
- Open access
- gold
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- Lin, Y., Wang, T., Zhang, L., Zhang, G., Li, L., Chang, Q., Pang, Z., Gao, H., Huang, K., Zhang, P., Zhao, Z.-J., Pei, C., & Gong, J. (2023). Tunable CO2 electroreduction to ethanol and ethylene with controllable interfacial wettability. Nature Communications. https://doi.org/10.1038/s41467-023-39351-2
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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