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Crystal phase-based epitaxial growth of hybrid noble metal nanostructures on 4H/fcc Au nanowires
Abstract
Crystal-phase engineering offers opportunities for the rational design and synthesis of noble metal nanomaterials with unusual crystal phases that normally do not exist in bulk materials. However, it remains a challenge to use these materials as seeds to construct heterometallic nanostructures with desired crystal phases and morphologies for promising applications such as catalysis. Here, we report a strategy for the synthesis of binary and ternary hybrid noble metal nanostructures. Our synthesized crystal-phase heterostructured 4H/fcc Au nanowires enable the epitaxial growth of Ru nanorods on the 4H phase and fcc-twin boundary in Au nanowires, resulting in hybrid Au-Ru nanowires. Moreover, the method can be extended to the epitaxial growth of Rh, Ru-Rh and Ru-Pt nanorods on the 4H/fcc Au nanowires to form unique hybrid nanowires. Importantly, the Au-Ru hybrid nanowires with tunable compositions exhibit excellent electrocatalytic performance towards the hydrogen evolution reaction in alkaline media.
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B-Os aerogels have Tafel slopes of approximately 26.8 and 44.7 mV dec−1 in 0.5 M H2SO4 and 1 M PBS, indicating more beneficial HER kinetics than Os NPs and Pt/C.
“The Tafel slopes of B-Os aerogels in 0.5 M H2SO4 and 1 M PBS were approximately 26.8 and 44.7 mV dec−1, indicating that the B-Os aerogel has the more beneficial HER kinetics than Os NPs and Pt/C”
From Interstitial boron-triggered electron-deficient Os aerogels for enhanced pH-universal hydrogen evolution (2022) · cites this paper as [50]
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Metadata
- Authors
- Lu, Q., Wang, A.-L., Gong, Y., Hao, W., Cheng, H., Chen, J., Li, B., Yang, N., Niu, W., Wang, J., Yu, Y., Zhang, X., Chen, Y., Fan, Z., Wu, X.-J., Chen, J., Luo, J., Li, S., Gu, L., & Zhang, H.
- Affiliations
- Nanyang Technological University (SG)
- Chinese Academy of Sciences (CN)
- Tianjin University of Technology (CN)
- Agency for Science, Technology and Research (SG)
- Corresponding author
- Gu, Lin
- Zhang, Hua
- ORCID
- Venue
- Nature Chemistry
- Published
- 2018-03-12
- Volume
- 10
- Issue
- 4
- Pages
- 456-461
- ISSN
- 1755-4330 (ISSN-L)
- 1755-4349
- OpenAlex
- W2790117439
- Cited by
- 301
- References
- 28
- Citations by year
- 2026: 18 · 2025: 26 · 2024: 36 · 2023: 30 · 2022: 43 · 2021: 52 · 2020: 39 · 2019: 40 · 2018: 17
- FWCI
- 8.53
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- www.springer.com/tdm (tdm)
- Locations
- Nature Chemistry (publishedVersion)
- PubMed (publishedVersion)
- DR-NTU (Nanyang Technological University) (submittedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Physical Sciences › Materials Science › Materials Chemistry › Copper-based nanomaterials and applications
- Keywords
- crystal phase engineering, epitaxial growth, hydrogen evolution reaction, electrocatalysis
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