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Ultrahigh-Gain Photodetectors Based on Atomically Thin Graphene-MoS2 Heterostructures

Open access
Zhang, Wenjing, Chuu, Chih-Piao, Huang, Jing-Kai, Chen, Chang-Hsiao, Tsai, Meng-Lin, Chang, Yung-Huang, Liang, Chi-Te, Chen, Yu-Ze, Chueh, Yu-Lun, He, Jr-Hau, Chou, Mei-Yin, Li, Lain-Jong·2014·Scientific Reports

Abstract

Due to its high carrier mobility, broadband absorption, and fast response time, the semi-metallic graphene is attractive for optoelectronics. Another two-dimensional semiconducting material molybdenum disulfide (MoS2) is also known as light- sensitive. Here we show that a large-area and continuous MoS2 monolayer is achievable using a CVD method and graphene is transferable onto MoS2. We demonstrate that a photodetector based on the graphene/MoS2 heterostructure is able to provide a high photogain greater than 10(8). Our experiments show that the electron-hole pairs are produced in the MoS2 layer after light absorption and subsequently separated across the layers. Contradictory to the expectation based on the conventional built-in electric field model for metal-semiconductor contacts, photoelectrons are injected into the graphene layer rather than trapped in MoS2 due to the presence of a perpendicular effective electric field caused by the combination of the built-in electric field, the applied electrostatic field, and charged impurities or adsorbates, resulting in a tuneable photoresponsivity.

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Metadata

Authors
Zhang, W., Chuu, C.-P., Huang, J.-K., Chen, C.-H., Tsai, M.-L., Chang, Y.-H., Liang, C.-T., Chen, Y.-Z., Chueh, Y.-L., He, J.-H., Chou, M.-Y., & Li, L.-J.
Venue
Scientific Reports
Published
2014-01-23
Volume
4
Issue
1
Pages
3826-3826
ISSN
2045-2322 (ISSN-L)
OpenAlex
W2067001296
Cited by
911
References
4
FWCI
58.22
Type
journal article
Language
en
Open access
gold

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CoChat. (2026). Citation check: Ultrahigh-Gain Photodetectors Based on Atomically Thin Graphene-MoS2 Heterostructures. https://app.cochat.ai/papers/10.1038/srep03826
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Zhang, W., Chuu, C.-P., Huang, J.-K., Chen, C.-H., Tsai, M.-L., Chang, Y.-H., Liang, C.-T., Chen, Y.-Z., Chueh, Y.-L., He, J.-H., Chou, M.-Y., & Li, L.-J. (2014). Ultrahigh-Gain Photodetectors Based on Atomically Thin Graphene-MoS2 Heterostructures. Scientific Reports. https://doi.org/10.1038/srep03826

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