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Gapless quantum spin liquid ground state in the two-dimensional spin-1/2 triangular antiferromagnet YbMgGaO4

Open access
Li, Yuesheng, Liao, Haijun, Zhang, Zhen, Li, Shiyan, Jin, Feng, Ling, Langsheng, Zhang, Lei, Zou, Youming, Pi, Li, Yang, Zhaorong, Wang, Junfeng, Wu, Zhonghua, Zhang, Qingming·2015·Scientific Reports

Abstract

Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in condensed matter physics. Here we report the successful synthesis of a new spin-1/2 triangular antiferromagnet YbMgGaO 4 with "Equation missing" sy m metry. The compound with an ideal two-dimensional and spatial isotropic magnetic triangular-lattice has no site-mixing magnetic defects and no antisymmetric Dzyaloshinsky-Moriya (DM) interactions. No spin freezing down to 60 mK (despite θ w ~ −4 K), the power-law temperature dependence of heat capacity and nonzero susceptibility at low temperatures suggest that YbMgGaO 4 is a promising gapless (≤|θ w|/100) QSL candidate. The residual spin entropy, which is accurately determined with a non-magnetic reference LuMgGaO 4, approaches zero (<0.6%). This indicates that the possible QSL ground state (GS) of the frustrated spin system has been experimentally achieved at the lowest measurement temperatures.

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Crossref · 10.1038/srep16419

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Metadata

Authors
Li, Y., Liao, H., Zhang, Z., Li, S., Jin, F., Ling, L., Zhang, L., Zou, Y., Pi, L., Yang, Z., Wang, J., Wu, Z., & Zhang, Q.
Venue
Scientific Reports
Published
2015-11-10
Volume
5
Issue
1
Pages
16419-16419
ISSN
2045-2322 (ISSN-L)
OpenAlex
W3105052732
Cited by
337
References
2
FWCI
9.75
Type
journal article
Language
en
Open access
gold

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