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Platinum dissolution and deposition in the polymer electrolyte membrane of a PEM fuel cell as studied by potential cycling
Abstract
The behavior of platinum dissolution and deposition in the polymer electrolyte membrane of a membrane-electrode-assembly (MEA) for a proton-exchange membrane fuel cell (PEMFC) was studied using potential cycling experiment and high-resolution transmission electron microscopy (HRTEM). The electrochemically active surface area decreased depending on the cycle number and the upper potential limit. Platinum deposition was observed in the polymer electrolyte membrane near a cathode catalyst layer. Platinum deposition was accelerated by the presence of hydrogen transported through the membrane from an anode compartment. Platinum was transported across the membrane and deposited on the anode layer in the absence of hydrogen in the anode compartment. This deposition was also affected by the presence of oxygen in the cathode compartment.
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Citations
Cites
Catalysis for Low Temperature Fuel Cells: PART I: THE CATHODE CHALLENGES
Ralph, T. R., & Hogarth, M. P. (2002) · Platinum Metals Review · doi:10.1595/003214002x461314 · Cited by 338
Cited by
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Cullen, D. A., Neyerlin, K. C., Ahluwalia, R. K., Mukundan, R., More, K. L., Borup, R. L., Weber, A. Z., Myers, D. J., & Kusoglu, A. (2021) · Nature Energy · doi:10.1038/s41560-021-00775-z · Cited by 1,277
Understanding and approaches for the durability issues of Pt-based catalysts for PEM fuel cell
Shao, Y., Yin, G., & Gao, Y. (2007) · Journal of Power Sources · doi:10.1016/j.jpowsour.2007.07.004 · Cited by 1,197
Ren, P., Pei, P., Li, Y., Wu, Z., Chen, D., & Huang, S. (2020) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2020.100859 · Cited by 737
Zatoń, M., Rozière, J., & Jones, D. J. (2017) · Sustainable Energy & Fuels · doi:10.1039/c7se00038c · Cited by 435
Chen, S., Gasteiger, H. A., Hayakawa, K., Tada, T., & Shao-Horn, Y. (2010) · Journal of The Electrochemical Society · doi:10.1149/1.3258275 · Cited by 360
Metadata
- Authors
- Yasuda, K., Taniguchi, A., Akita, T., Ioroi, T., & Siroma, Z.
- Venue
- Phys. Chem. Chem. Phys.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2006
- Volume
- 8
- Issue
- 6
- Pages
- 746-752
- ISSN
- 1463-9076 (ISSN-L)
- 1463-9084
- OpenAlex
- W2010576058
- Cited by
- 376
- References
- 1
- FWCI
- 13.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yasuda, K., Taniguchi, A., Akita, T., Ioroi, T., & Siroma, Z. (2006). Platinum dissolution and deposition in the polymer electrolyte membrane of a PEM fuel cell as studied by potential cycling. Phys. Chem. Chem. Phys. https://doi.org/10.1039/b514342j
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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