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Dynamic combinatorial chemistry: on the road to fulfilling the promise
Abstract
Dynamic combinatorial chemistry makes use of reversible reactions between functionalised monomeric building blocks to generate a mixture of products (dimers or oligomers) under thermodynamic equilibrium. This system reorganises upon addition of a target so that species that bind to, and are therefore stabilised by the target, are favourably formed and are thus amplified. Since the mid-1990's, dynamic combinatorial chemistry has been successfully applied to the identification/selection of ion receptors, enzyme inhibitors, catalysts, materials and nucleic acid ligands. Although it is now established as a powerful tool with broad applications some intrinsic limitations appeared when working on systems of increasing complexity. We present here the most recent advances in the field of dynamic combinatorial chemistry that have been developed to overcome these limitations and explore new areas of application.
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Cites
A chiroselective peptide replicator
Saghatelian, A., Yokobayashi, Y., Soltani, K., & Ghadiri, M. R. (2001) · Nature · doi:10.1038/35057238 · Cited by 310
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Prebiotic Systems Chemistry: New Perspectives for the Origins of Life
Ruiz-Mirazo, K., Briones, C., & de la Escosura, A. (2014) · Chemical Reviews · doi:10.1021/cr2004844 · Cited by 930
Herrmann, A. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60336a · Cited by 351
Dynamic Diselenide Bonds: Exchange Reaction Induced by Visible Light without Catalysis
Ji, S., Cao, W., Yu, Y., & Xu, H. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201403442 · Cited by 337
Evolution of Dynamic Combinatorial Chemistry
Cougnon, F. B. L., & Sanders, J. K. M. (2012) · Accounts of Chemical Research · doi:10.1021/ar200240m · Cited by 316
Metadata
- Authors
- Ladame, S.
- Venue
- Org. Biomol. Chem.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2008
- Volume
- 6
- Issue
- 2
- Pages
- 219-226
- ISSN
- 1477-0520 (ISSN-L)
- 1477-0539
- OpenAlex
- W2042931146
- Cited by
- 242
- References
- 1
- FWCI
- 11.98
- Type
- journal article
- Language
- en
- Open access
- closed
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