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Composite photoanodes for photoelectrochemical solar water splitting

Sun, Jianwei, Zhong, Diane K., Gamelin, Daniel R.·2010·Energy & Environmental Science
DOI 10.1039/c0ee00030b
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Abstract

Photoelectrochemical (PEC) water splitting is an attractive approach to capturing and storing the earth's abundant solar energy influx. The challenging four-electron water-oxidation half-cell reaction has hindered this technology, giving rise to slow water oxidation kinetics at the photoanode surfaces relative to competitive loss processes. In this perspective, we review recent efforts to improve PEC efficiencies by modification of semiconductor photoanode surfaces with water-oxidation catalysts that can operate at low overpotentials. This approach allows separation of the tasks of photon absorption, charge separation, and surface catalysis, allowing each to be optimized independently. In particular, composite photoanodes marrying nanocrystalline and molecular/non-crystalline components provide flexibility in adjusting the properties of each component, but raise new challenges in interfacial chemistries.

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Metadata

Authors
Sun, J., Zhong, D. K., & Gamelin, D. R.
Venue
Energy & Environmental Science
Publisher
Royal Society of Chemistry (RSC)
Published
2010
Volume
3
Issue
9
Pages
1252
ISSN
  • 1754-5692 (ISSN-L)
  • 1754-5706
DOI
10.1039/c0ee00030b
OpenAlex
W2072758315
Cited by
281
References
1
FWCI
9.78
Type
journal article
Language
en
Open access
closed

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CoChat. (2026). Citation check: Composite photoanodes for photoelectrochemical solar water splitting. https://app.cochat.ai/papers/10.1039/c0ee00030b
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Sun, J., Zhong, D. K., & Gamelin, D. R. (2010). Composite photoanodes for photoelectrochemical solar water splitting. Energy & Environmental Science. https://doi.org/10.1039/c0ee00030b

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