The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
N-Heterocyclic carbene functionalized MCM-41 as an efficient catalyst for chemical fixation of carbon dioxide
Abstract
N-Heterocyclic carbene (NHC) functionalized MCM-41 was synthesized by reacting 1,3-bis-(4-allyl-2,6-diisopropylphenyl) imidazolium chloride with MCM-41 using 3-mercaptopropyltrimethoxysilane as silane coupling agent, and its CO2 adduct (designated as MCM-41-IPr-CO2) was further synthesized by the reaction with CO2. In situdiffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) was used to investigate the reversible CO2 capture-release ability of MCM-41-NHC. MCM-41-IPr-CO2 adduct proved to be an efficient heterogeneous catalyst for the cycloaddition of CO2 to epoxides or aziridines with excellent regioselectivity under mild conditions. Moreover, the catalyst could be recovered easily through a simple filtration process and reused multiple times without obvious loss in activity, owing to CO2 as protective group for effectively stabilizing the NHC anchored on MCM-41.
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Cites
Darensbourg, D. J. (2007) · Chemical Reviews · doi:10.1021/cr068363q · Cited by 1,593
Shaikh, A.-A. G., & Sivaram, S. (1996) · Chemical Reviews · doi:10.1021/cr950067i · Cited by 1,381
Reactive Applications of Cyclic Alkylene Carbonates
Clements, J. H. (2003) · Industrial & Engineering Chemistry Research · doi:10.1021/ie020678i · Cited by 784
Cited by
Shaikh, R. R., Pornpraprom, S., & D’Elia, V. (2018) · ACS Catalysis · doi:10.1021/acscatal.7b03580 · Cited by 729
Sustainable conversion of carbon dioxide: the advent of organocatalysis
Fiorani, G., Guo, W., & Kleij, A. W. (2015) · Green Chemistry · doi:10.1039/c4gc01959h · Cited by 658
Alves, M., Grignard, B., Mereau, R., Jerome, C., Tassaing, T., & Detrembleur, C. (2017) · Catalysis Science & Technology · doi:10.1039/c7cy00438a · Cited by 531
Recent progress in catalytic conversions of carbon dioxide
Maeda, C., Miyazaki, Y., & Ema, T. (2014) · Catalysis Science & Technology · doi:10.1039/c3cy00993a · Cited by 517
Ema, T., Miyazaki, Y., Shimonishi, J., Maeda, C., & Hasegawa, J.-Y. (2014) · Journal of the American Chemical Society · doi:10.1021/ja507665a · Cited by 473
Metadata
- Authors
- Zhou, H., Wang, Y.-M., Zhang, W.-Z., Qu, J.-P., & Lu, X.-B.
- Venue
- Green Chemistry
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 13
- Issue
- 3
- Pages
- 644
- ISSN
- 1463-9262 (ISSN-L)
- 1463-9270
- OpenAlex
- W1987449170
- Cited by
- 191
- References
- 3
- FWCI
- 9.89
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhou, H., Wang, Y.-M., Zhang, W.-Z., Qu, J.-P., & Lu, X.-B. (2011). N-Heterocyclic carbene functionalized MCM-41 as an efficient catalyst for chemical fixation of carbon dioxide. Green Chemistry. https://doi.org/10.1039/c0gc00541j
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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