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Electrocatalytic reduction of CO2 to CO by polypyridyl ruthenium complexes
Abstract
Electrocatalytic reduction of CO(2) by [Ru(tpy)(bpy)(solvent)](2+) (tpy = 2,2':6',2''-terpyridine, bpy = 2,2'-bipyridine) and its structural analogs is initiated by sequential 1e(-) reductions at the tpy and bpy ligands followed by rate limiting CO(2) addition to give a metallocarboxylate intermediate. It undergoes further reduction and loss of CO.
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Citations
Cited by
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
Frontiers, Opportunities, and Challenges in Biochemical and Chemical Catalysis of CO 2 Fixation
Appel, A. M., Bercaw, J. E., Bocarsly, A. B., Dobbek, H., DuBois, D. L., Dupuis, M., Ferry, J. G., Fujita, E., Hille, R., Kenis, P. J. A., et al. (2013) · Chemical Reviews · doi:10.1021/cr300463y · Cited by 2,193
A Local Proton Source Enhances CO 2 Electroreduction to CO by a Molecular Fe Catalyst
Costentin, C., Drouet, S., Robert, M., & Savéant, J.-M. (2012) · Science · doi:10.1126/science.1224581 · Cited by 1,315
Molecular polypyridine-based metal complexes as catalysts for the reduction of CO2
Elgrishi, N., Chambers, M. B., Wang, X., & Fontecave, M. (2017) · Chemical Society Reviews · doi:10.1039/c5cs00391a · Cited by 555
Advances in molecular photocatalytic and electrocatalytic CO2 reduction
Windle, C. D., & Perutz, R. N. (2012) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2012.03.010 · Cited by 481
Metadata
- Authors
- Chen, Z., Chen, C., Weinberg, D. R., Kang, P., Concepcion, J. J., Harrison, D. P., Brookhart, M. S., & Meyer, T. J.
- Venue
- Chemical Communications
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 47
- Issue
- 47
- Pages
- 12607
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W2009184234
- Cited by
- 237
- References
- 0
- FWCI
- 7.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chen, Z., Chen, C., Weinberg, D. R., Kang, P., Concepcion, J. J., Harrison, D. P., Brookhart, M. S., & Meyer, T. J. (2011). Electrocatalytic reduction of CO2 to CO by polypyridyl ruthenium complexes. Chemical Communications. https://doi.org/10.1039/c1cc15071e
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