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Structural investigations into the deactivation pathway of the CO2 reduction electrocatalyst Re(bpy)(CO)3Cl
Abstract
We report a series of complexes synthesized from the chemical reduction of the fac-tricarbonyl complex Re(bpy)(CO)(3)Cl. Synthesis and characterization of [Re(bpy)(CO)(3)](2), [Re(bpy)(CO)(3)](2)(-), and Re(bpy)(CO)(3)(-) are presented. The Re(bpy)(CO)(3)(-) anion has long been postulated as the active species that reacts with carbon dioxide in the electrochemical reduction of CO(2).
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Cited by
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
Plasmon-Enhanced Photocatalytic CO2 Conversion within Metal–Organic Frameworks under Visible Light
Choi, K. M., Kim, D., Rungtaweevoranit, B., Trickett, C. A., Barmanbek, J. T. D., Alshammari, A. S., Yang, P., & Yaghi, O. M. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.6b11027 · Cited by 632
Molecular polypyridine-based metal complexes as catalysts for the reduction of CO2
Elgrishi, N., Chambers, M. B., Wang, X., & Fontecave, M. (2017) · Chemical Society Reviews · doi:10.1039/c5cs00391a · Cited by 555
Sampson, M. D., Nguyen, A. D., Grice, K. A., Moore, C. E., Rheingold, A. L., & Kubiak, C. P. (2014) · Journal of the American Chemical Society · doi:10.1021/ja501252f · Cited by 466
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Metadata
- Authors
- Benson, E. E., & Kubiak, C. P.
- Venue
- Chemical Communications
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2012
- Volume
- 48
- Issue
- 59
- Pages
- 7374
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W2139978094
- Cited by
- 162
- References
- 0
- FWCI
- 4.37
- Type
- journal article
- Language
- en
- Open access
- closed
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- Benson, E. E., & Kubiak, C. P. (2012). Structural investigations into the deactivation pathway of the CO2 reduction electrocatalyst Re(bpy)(CO)3Cl. Chemical Communications. https://doi.org/10.1039/c2cc32617e
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