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Creating, characterizing, and controlling chemistry with SERS hot spots
Abstract
In this perspective we discuss the roles of hot spots in surface-enhanced Raman spectroscopy (SERS). After giving background and defining the hot spot, we evaluate a variety of SERS substrates which often contain hot spots. We compare and discuss the differentiating properties of each substrate. We then provide a thorough analysis of the hot spot contribution to the observed SERS signal both in ensemble-averaged and single-molecule conditions. We also enumerate rules for determining the SERS enhancement factor (EF) to clarify the use of this common metric. Finally, we present a forward-looking overview of applications and uses of hot spots for controlling chemistry on the nanoscale. Although not exhaustive, this perspective is a review of some of the most interesting and promising methodologies for creating, controlling, and using hot spots for electromagnetic amplification.
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Citations
Cites
Surface raman spectroelectrochemistry
Jeanmaire, D. L., & Van Duyne, R. P. (1977) · Journal of Electroanalytical Chemistry and Interfacial Electrochemistry · doi:10.1016/s0022-0728(77)80224-6 · Cited by 4,738
Cited by
Fundamental understanding and applications of plasmon-enhanced Raman spectroscopy
Wang, X., Huang, S.-C., Hu, S., Yan, S., & Ren, B. (2020) · Nature Reviews Physics · doi:10.1038/s42254-020-0171-y · Cited by 689
Large-Scale Hot Spot Engineering for Quantitative SERS at the Single-Molecule Scale
Chen, H.-Y., Lin, M.-H., Wang, C.-Y., Chang, Y.-M., & Gwo, S. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b09111 · Cited by 426
Infrared and Raman chemical imaging and spectroscopy at the nanoscale
Kurouski, D., Dazzi, A., Zenobi, R., & Centrone, A. (2020) · Chemical Society Reviews · doi:10.1039/c8cs00916c · Cited by 324
In Vitro and In Vivo SERS Biosensing for Disease Diagnosis
Moore, T. J., Moody, A. S., Payne, T. D., Sarabia, G. M., Daniel, A. R., & Sharma, B. (2018) · Biosensors · doi:10.3390/bios8020046 · Cited by 161
The substrate matters in the Raman spectroscopy analysis of cells
Mikoliunaite, L., Rodriguez, R. D., Sheremet, E., Kolchuzhin, V., Mehner, J., Ramanavicius, A., & Zahn, D. R. T. (2015) · Scientific Reports · doi:10.1038/srep13150 · Cited by 87
Metadata
- Authors
- Kleinman, S. L., Frontiera, R. R., Henry, A.-I., Dieringer, J. A., & Van Duyne, R. P.
- Venue
- Phys. Chem. Chem. Phys.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 15
- Issue
- 1
- Pages
- 21-36
- ISSN
- 1463-9076 (ISSN-L)
- 1463-9084
- OpenAlex
- W2093468996
- Cited by
- 733
- References
- 1
- FWCI
- 19.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kleinman, S. L., Frontiera, R. R., Henry, A.-I., Dieringer, J. A., & Van Duyne, R. P. (2013). Creating, characterizing, and controlling chemistry with SERS hot spots. Phys. Chem. Chem. Phys. https://doi.org/10.1039/c2cp42598j
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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