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Efficient and stable CH3NH3PbI3-sensitized ZnO nanorod array solid-state solar cells
Open accessAbstract
We report for the first time the use of a perovskite (CH3NH3PbI3) absorber in combination with ZnO nanorod arrays (NRAs) for solar cell applications. The perovskite material has a higher absorption coefficient than molecular dye sensitizers, gives better solar cell stability, and is therefore more suited as a sensitizer for ZnO NRAs. A solar cell efficiency of 5.0% was achieved under 1000 W m(-2) AM 1.5 G illumination for a solar cell with the structure: ZnO NRA/CH3NH3PbI3/spiro-MeOTAD/Ag. Moreover, the solar cell shows a good long-term stability. Using transient photocurrent and photovoltage measurements it was found that the electron transport time and lifetime vary with the ZnO nanorod length, a trend which is similar to that in dye-sensitized solar cells, DSCs, suggesting a similar charge transfer process in ZnO NRA/CH3NH3PbI3 solar cells as in conventional DSCs. Compared to CH3NH3PbI3/TiO2 solar cells, ZnO shows a lower performance due to more recombination losses.
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Cites
Kim, H.-S., Lee, C.-R., Im, J.-H., Lee, K.-B., Moehl, T., Marchioro, A., Moon, S.-J., Humphry-Baker, R., Yum, J.-H., Moser, J. E., et al. (2012) · Scientific Reports · doi:10.1038/srep00591 · Cited by 8,092
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Yu, Z., & Sun, L. (2015) · Advanced Energy Materials · doi:10.1002/aenm.201500213 · Cited by 462
p-type Mesoscopic Nickel Oxide/Organometallic Perovskite Heterojunction Solar Cells
Wang, K.-C., Jeng, J.-Y., Shen, P.-S., Chang, Y.-C., Diau, E. W.-G., Tsai, C.-H., Chao, T.-Y., Hsu, H.-C., Lin, P.-Y., Chen, P., et al. (2014) · Scientific Reports · doi:10.1038/srep04756 · Cited by 444
Device stability of perovskite solar cells – A review
Asghar, M. I., Zhang, J., Wang, H., & Lund, P. D. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.04.003 · Cited by 423
Liang, P., Chueh, C., Williams, S. T., & Jen, A. K. ‐. (2015) · Advanced Energy Materials · doi:10.1002/aenm.201402321 · Cited by 353
Metadata
- Authors
- Bi, D., Boschloo, G., Schwarzmüller, S., Yang, L., Johansson, E. M. J., & Hagfeldt, A.
- Venue
- Nanoscale
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 5
- Issue
- 23
- Pages
- 11686
- ISSN
- 2040-3364 (ISSN-L)
- 2040-3372
- OpenAlex
- W2168557397
- Cited by
- 281
- References
- 1
- FWCI
- 26.36
- Type
- journal article
- Language
- en
- Open access
- green
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- Bi, D., Boschloo, G., Schwarzmüller, S., Yang, L., Johansson, E. M. J., & Hagfeldt, A. (2013). Efficient and stable CH3NH3PbI3-sensitized ZnO nanorod array solid-state solar cells. Nanoscale. https://doi.org/10.1039/c3nr01542d
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