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Synthesis and crystal chemistry of the hybrid perovskite (CH3NH3)PbI3 for solid-state sensitised solar cell applications
Open accessAbstract
The hybrid organic–inorganic perovskite (CH3NH3)PbI3 may find application in next generation solid-state sensitised solar cells. Although this material and related perovskites were discovered many decades ago, questions remain concerning their diverse structural chemistry and unusual properties. The article presents a review of previous work and provides a detailed description of the preparation, structural characterisation and physical characteristics of (CH3NH3)PbI3. The phase changes exhibited by (CH3NH3)PbI3 have been probed using variable temperature powder and single crystal X-ray diffraction, combined with differential scanning calorimetry, thermogravimetric analysis and phase contrast transmission electron microscopy. The optical band gap for (CH3NH3)PbI3 determined by UV-Visible spectroscopy was compared to values obtained from density-of-state simulation of the electronic band structure.
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Cites
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Cited by
Saidaminov, M. I., Abdelhady, A. L., Murali, B., Alarousu, E., Burlakov, V. M., Peng, W., Dursun, I., Wang, L., He, Y., Maculan, G., et al. (2015) · Nature Communications · doi:10.1038/ncomms8586 · Cited by 1,922
Excitons versus free charges in organo-lead tri-halide perovskites
D’Innocenzo, V., Grancini, G., Alcocer, M. J. P., Kandada, A. R. S., Stranks, S. D., Lee, M. M., Lanzani, G., Snaith, H. J., & Petrozza, A. (2014) · Nature Communications · doi:10.1038/ncomms4586 · Cited by 1,767
Brenner, T. M., Egger, D. A., Kronik, L., Hodes, G., & Cahen, D. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.7 · Cited by 1,557
Depleted hole conductor-free lead halide iodide heterojunction solar cells
Laban, W. A., & Etgar, L. (2013) · Energy & Environmental Science · doi:10.1039/c3ee42282h · Cited by 759
Organolead Halide Perovskite: New Horizons in Solar Cell Research
Kim, H.-S., Im, S. H., & Park, N.-G. (2014) · The Journal of Physical Chemistry C · doi:10.1021/jp409025w · Cited by 722
Metadata
- Authors
- Baikie, T., Fang, Y., Kadro, J. M., Schreyer, M., Wei, F., Mhaisalkar, S. G., Graetzel, M., & White, T. J.
- Venue
- Journal of Materials Chemistry A
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 1
- Issue
- 18
- Pages
- 5628
- ISSN
- 2050-7488 (ISSN-L)
- 2050-7496
- OpenAlex
- W2171105325
- Cited by
- 2,534
- References
- 3
- FWCI
- 147.38
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Baikie, T., Fang, Y., Kadro, J. M., Schreyer, M., Wei, F., Mhaisalkar, S. G., Graetzel, M., & White, T. J. (2013). Synthesis and crystal chemistry of the hybrid perovskite (CH3NH3)PbI3 for solid-state sensitised solar cell applications. Journal of Materials Chemistry A. https://doi.org/10.1039/c3ta10518k
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