Cited by 294Polymer composites and self-healingAdvanced Materials and MechanicsHydrogels: synthesis, properties, applications

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Water-induced shape memory effect of graphene oxide reinforced polyvinyl alcohol nanocomposites

Qi, Xiaodong, Yao, Xuelin, Deng, Sha, Zhou, Tiannan, Fu, Qiang·2014·J. Mater. Chem. A

DOI 10.1039/c3ta14340f

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Abstract

A novel water-induced shape memory polymer based on polyvinyl alcohol (PVA) was prepared by introducing graphene oxide (GO). Due to the strong hydrogen bonding interaction between PVA and GO, some additional physically cross-linked points could be formed in PVA, which largely improved shape memory properties of PVA. Solvent-induced shape memory behavior was observed by immersing PVA/GO nanocomposites in water. The water-induced shape recovery was due to the decrease of glass transition temperature and storage modulus. This could be explained by the swelling plasticizing effect of water on PVA, as indicated by the obvious expansion in volume of PVA. On the other hand, the weakened hydrogen bonding between PVA and GO was also observed after immersing the PVA/GO nanocomposites in water. Thus both the plasticizing effect and the competitive hydrogen bonding were the two main reasons for the shape recovery of PVA/GO nanocomposites. This study provides a framework for developing new shape memory polymers (SMPs) and for better understanding the shape recovery mechanism in solvent-induced SMPs.

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Authors: Qi, X., Yao, X., Deng, S., Zhou, T., & Fu, Q.
Affiliations: Sichuan University (CN)
Corresponding author: Fu, Qiang
ORCID: Yao, Xuelin
Deng, Sha
Fu, Qiang
Venue: J. Mater. Chem. A
Publisher: Royal Society of Chemistry (RSC)
Published: 2014
Volume: 2
Issue: 7
Pages: 2240-2249
ISSN: 2050-7488 (ISSN-L)
2050-7496
DOI: 10.1039/c3ta14340f
OpenAlex: W2107642160
Cited by: 293
References: 47
Citations by year: 2026: 6 · 2025: 12 · 2024: 13 · 2023: 11 · 2022: 23 · 2021: 33 · 2020: 26 · 2019: 36 · 2018: 31 · 2017: 36 · 2016: 38 · 2015: 19 · 2014: 8
FWCI: 15.65
Type: journal article
Language: en
Open access: closed
Locations: Journal of Materials Chemistry A (publishedVersion)
Topics: Physical Sciences › Materials Science › Polymers and Plastics › Polymer composites and self-healing
Physical Sciences › Engineering › Mechanical Engineering › Advanced Materials and Mechanics
Physical Sciences › Materials Science › Biomaterials › Hydrogels: synthesis, properties, applications
Keywords: shape memory polymers, polyvinyl alcohol, graphene oxide, polymer nanocomposites, hydrogen bonding, physical crosslinking, water swelling, plasticization, glass transition temperature, storage modulus

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Water-induced shape memory effect of graphene oxide reinforced polyvinyl alcohol nanocomposites

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