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Incorporation of iron hydrogenase active sites into a highly stable metal–organic framework for photocatalytic hydrogen generation
Abstract
A new biomimetic heterogeneous photocatalyst ([FeFe]@ZrPF) has been synthesized through the incorporation of homogeneous complex 1 [(í-SCH2)2NC(O)C5H4N]-[Fe2(CO)6] into the highly robust zirconium-porphyrin based metal-organic framework (ZrPF). The immobilized biomimetic [Fe2S2] catalyst inside the MOF shows great improvement in hydrogen generation compared to the reference homogeneous catalyst complex 1.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Photosynthetic energy conversion: natural and artificial
Barber, J. (2009) · Chem. Soc. Rev. · doi:10.1039/b802262n · Cited by 1,843
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Nanomaterials with enzyme-like characteristics (nanozymes): next-generation artificial enzymes
Wei, H., & Wang, E. (2013) · Chemical Society Reviews · doi:10.1039/c3cs35486e · Cited by 3,779
Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
Single Pt Atoms Confined into a Metal–Organic Framework for Efficient Photocatalysis
Fang, X., Shang, Q., Wang, Y., Jiao, L., Yao, T., Li, Y., Zhang, Q., Luo, Y., & Jiang, H. (2018) · Advanced Materials · doi:10.1002/adma.201705112 · Cited by 837
Metadata
- Authors
- Sasan, K., Lin, Q., Mao, C., & Feng, P.
- Venue
- Chemical Communications
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2014-07-25
- Volume
- 50
- Issue
- 72
- Pages
- 10390
- ISSN
- 1359-7345 (ISSN-L)
- 1364-548X
- OpenAlex
- W2025884393
- Cited by
- 193
- References
- 2
- FWCI
- 5.35
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sasan, K., Lin, Q., Mao, C., & Feng, P. (2014). Incorporation of iron hydrogenase active sites into a highly stable metal–organic framework for photocatalytic hydrogen generation. Chemical Communications. https://doi.org/10.1039/c4cc03946g
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
