High oxygen-reduction activity and durability of nitrogen-doped graphene
Abstract
Nitrogen-doped graphene as a metal-free catalyst for oxygen reduction was synthesized by heat-treatment of graphene using ammonia. It was found that the optimum temperature was 900 °C. The resulting catalyst had a very high oxygen reduction reaction (ORR) activity through a four-electron transfer process in oxygen-saturated 0.1 M KOH. Most importantly, the electrocatalytic activity and durability of this material are comparable or better than the commercial Pt/C (loading: 4.85 µgPt cm−2). XPS characterization of these catalysts was tested to identify the active N species for ORR.
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Once Pt loading is decreased, the number of available active sites is also decreased, thus leading to severe performance loss.
“However, once Pt loading is decreased, the number of available active sites is also decreased, thus leading to severe performance loss [238,239].”
From Recent Advances on PEM Fuel Cells: From Key Materials to Membrane Electrode Assembly (2023) · cites this paper as [239]
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- Authors
- Geng, D., Chen, Y., Chen, Y., Li, Y., Li, R., Sun, X., Ye, S., & Knights, S.
- Affiliations
- Western University (CA)
- Ballard Power Systems (Canada) (CA)
- Corresponding author
- Sun, Xueliang
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2011
- Volume
- 4
- Issue
- 3
- Pages
- 760
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W1999469559
- Cited by
- 1,219
- References
- 29
- Citations by year
- 2026: 10 · 2025: 23 · 2024: 34 · 2023: 26 · 2022: 47 · 2021: 53 · 2020: 71 · 2019: 121 · 2018: 132 · 2017: 133 · 2016: 132 · 2015: 147 · 2014: 122 · 2013: 94 · 2012: 60
- FWCI
- 38.58
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Energy & Environmental Science (publishedVersion)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
- Keywords
- nitrogen-doped graphene, oxygen reduction reaction, metal-free electrocatalysts, ammonia treatment, heat treatment temperature, four-electron pathway, Pt/C comparison, alkaline electrolyte
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