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Aggregate-based sub-CMC solubilization of hexadecane by surfactants
Abstract
SDBS or Triton X-100 at sub-CMC concentrations enhances hexadecane solubilization due to the aggregate formation mechanism. The sub-CMC aggregate size decreases with increasing surface excess of the surfactant.
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Two proposed mechanisms for solubilization observed below the surfactant CMC are the reduction in NAPL-water interfacial tension and the formation of pre-micellar aggregates.
“Two proposed mechanisms for solubilization observed below the surfactant CMC are the reduction in NAPL-water interfacial tension and the formation of pre-micellar aggregates (e.g., refs 51–54).”
From Contribution of Nonaqueous-Phase Liquids to the Retention and Transport of Per and Polyfluoroalkyl Substances (PFAS) in Porous Media (2021) · cites this paper as [53]
The Conclusion and Results and discussion §4.4 attribute sub-CMC hexadecane solubilization to aggregate formation. Results and discussion §4.1 also documents reduced hexadecane–water interfacial tension as surfactant concentration rises, but the paper does not propose that reduction as a separate mechanism for the observed solubilization. (LLM, conf=0.85)
Experimental — accuracy not yet measuredMany studies have observed increased NAPL solubilization in the presence of surfactants.
“Many studies have observed increased NAPL solubilization in the presence of surfactants.”
From Contribution of Nonaqueous-Phase Liquids to the Retention and Transport of Per and Polyfluoroalkyl Substances (PFAS) in Porous Media (2021) · cites this paper as [53]
In other studies, solubilization was also observed when surfactant concentrations were below the CMC.
“Conversely, in other studies solubilization was also observed when surfactant concentrations were below the CMC (e.g., refs 50–54).”
From Contribution of Nonaqueous-Phase Liquids to the Retention and Transport of Per and Polyfluoroalkyl Substances (PFAS) in Porous Media (2021) · cites this paper as [53]
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Self-citation
Metadata
- Authors
- Zhong, H., Yang, L., Zeng, G., Brusseau, M. L., Wang, Y., Li, Y., Liu, Z., Yuan, X., & Tan, F.
- Venue
- RSC Advances
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2015
- Volume
- 5
- Issue
- 95
- Pages
- 78142-78149
- ISSN
- 2046-2069
- PMC
- PMC4765384
- Cited by
- 40
- References
- 0
- Language
- en
- Funders
- National Institute of Environmental Health Sciences (ES04940)
- National Natural Science Foundation of China (51108166, 51308200, 51378190, 51378192)
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