Stimulated X-ray Raman scattering – a critical assessment of the building block of nonlinear X-ray spectroscopy
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With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.
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Post-sorting the pair of pulses according to their total pulse energy and electron-beam energy resulted in very stable, reproducible spectral averages, so that relative differences of greater than 5% are measurable using this pulse combination.
“We, however, demonstrated that post-sorting the pair of pulses according to their total pulse energy and the electron-beam energy resulted in very stable, reproducible spectral averages, so that relative differences of >5% are measurable using this pulse combination [63].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [63]
Unaligned molecular targets at currently obtainable peak brilliances will give rise to soft x-ray Raman amplification of only a few per cent.
“As opposed to the studies in neon, where a Raman gain of up to eight orders of magnitude has been demonstrated [59], unaligned molecular targets at currently obtainable peak brilliances will give rise to soft x-ray Raman amplification of only a few per cent [62,63].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [63]
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Stohr, J. (2026) · Springer tracts in modern physics · doi:10.1007/978-3-032-07634-2_10
- Authors
- Kimberg, V., Sanchez-Gonzalez, A., Mercadier, L., Weninger, C., Lutman, A., Ratner, D., Coffee, R., Bucher, M., Mucke, M., Agåker, M., Såthe, C., Bostedt, C., Nordgren, J., Rubensson, J. E., & Rohringer, N.
- Affiliations
- Max Planck Institute for the Structure and Dynamics of Matter (DE)
- Imperial College
- SLAC National Accelerator Laboratory (US)
- Argonne National Laboratory (US)
- Uppsala University (SE)
- Corresponding author
- Kimberg, Victor
- Rohringer, Nina
- ORCID
- Venue
- Faraday Discussions
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2016
- Volume
- 194
- Pages
- 305-324
- ISSN
- 1359-6640 (ISSN-L)
- 1364-5498
- OpenAlex
- W2421283582
- Cited by
- 32
- References
- 28
- Citations by year
- 2026: 2 · 2025: 3 · 2024: 3 · 2023: 5 · 2022: 2 · 2021: 2 · 2020: 3 · 2019: 2 · 2018: 4 · 2017: 5 · 2016: 1
- FWCI
- 1.89
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- cc-by-nc
- Locations
- Faraday Discussions (publishedVersion, cc-by-nc)
- PubMed (publishedVersion)
- Desy Publications Database (Deutsches Elektronen-Synchrotron DESY) (submittedVersion, other-oa)
- MPG.PuRe (Max Planck Society) (submittedVersion, cc-by-nc)
- KTH Publication Database DiVA (KTH Royal Institute of Technology) (submittedVersion, other-oa)
- Max Planck Digital Library (submittedVersion, other-oa)
- DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron)
- Funders
- Vetenskapsrådet
- Max-Planck-Gesellschaft
- Knut och Alice Wallenbergs Stiftelse (KAW-2013.0020)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Keywords
- X-ray free-electron laser, femtosecond X-ray pulses, coherent electron dynamics, time-resolved X-ray spectroscopy
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