Stimulated Electronic X-Ray Raman Scattering
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We demonstrate strong stimulated inelastic x-ray scattering by resonantly exciting a dense gas target of neon with femtosecond, high-intensity x-ray pulses from an x-ray free-electron laser (XFEL). A small number of lower energy XFEL seed photons drive an avalanche of stimulated resonant inelastic x-ray scattering processes that amplify the Raman scattering signal by several orders of magnitude until it reaches saturation. Despite the large overall spectral width, the internal spiky structure of the XFEL spectrum determines the energy resolution of the scattering process in a statistical sense. This is demonstrated by observing a stochastic line shift of the inelastically scattered x-ray radiation. In conjunction with statistical methods, XFELs can be used for stimulated resonant inelastic x-ray scattering, with spectral resolution smaller than the natural width of the core-excited, intermediate state.
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Amplified spontaneous x-ray emission and stimulated resonant inelastic x-ray Raman scattering have been demonstrated in atomic Ne in the soft x-ray spectral range.
“Despite the ultrahigh intensities necessary for realizing stimulated x-ray emission (10 17 -10 18 W cm -2 in the soft and 10 19 -10 20 W cm -2 in the hard x-ray range), amplified spontaneous x-ray emission [58] and stimulated resonant inelastic x-ray Raman scattering (sRIXS) [59] have been demonstrated in atomic Ne in the soft x-ray spectral range.”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [59]
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- See Supplemental Material at http://link.aps.org/ supplemental/10.1103/PhysRevLett.111.233902 for the estimate of the absolute signal strength, calibration of the XFEL central photon energy, a summary of the theoretical approach and a discussion of the role of the XFEL as seed for the inelastic scattering process.
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- Authors
- Weninger, C., Purvis, M., Ryan, D., London, R. A., Bozek, J. D., Bostedt, C., Graf, A., Brown, G., Rocca, J. J., & Rohringer, N.
- Affiliations
- Max Planck Institute for the Physics of Complex Systems (DE)
- Colorado State University (US)
- Lawrence Livermore National Laboratory (US)
- SLAC National Accelerator Laboratory (US)
- ORCID
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2013-12-05
- Volume
- 111
- Issue
- 23
- Pages
- 233902-233902
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2032189197
- Cited by
- 148
- References
- 49
- Citations by year
- 2026: 4 · 2025: 9 · 2024: 13 · 2023: 12 · 2022: 9 · 2021: 16 · 2020: 14 · 2019: 14 · 2018: 9 · 2017: 3 · 2016: 13 · 2015: 23 · 2014: 9
- FWCI
- 7.72
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron) (submittedVersion, other-oa)
- Max Planck Institute for Plasma Physics (submittedVersion)
- Max Planck Digital Library (submittedVersion, other-oa)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Funders
- U.S. Department of Energy (DEAC5207NA27344, AC52‐07NA27344, Contract No. DE-AC52-07NA27344, No. DE-AC52-07NA27344)
- Office of Science (DE-AC52-07NA27344)
- Basic Energy Sciences (DE-AC52-07NA27344.)
- Lawrence Livermore National Laboratory (DE‐AC5207NA27344, No. DE-AC52-07NA27344, AC52-07NA27344)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Keywords
- stimulated Raman scattering, X-ray free-electron laser, neon gas, femtosecond X-ray pulses, signal amplification, spectral resolution, core-excited states, intermediate state, line shift, statistical analysis
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