Cited by 753CO2 Sequestration and Geologic InteractionsCarbon Dioxide Capture TechnologiesGeological and Geochemical Analysis

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In situ carbonation of peridotite for CO 2 storage

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Kelemen, Peter B., Matter, Jürg·2008·Proceedings of the National Academy of Sciences

DOI 10.1073/pnas.0805794105PMC PMC2582290

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Abstract

The rate of natural carbonation of tectonically exposed mantle peridotite during weathering and low-temperature alteration can be enhanced to develop a significant sink for atmospheric CO 2 . Natural carbonation of peridotite in the Samail ophiolite, an uplifted slice of oceanic crust and upper mantle in the Sultanate of Oman, is surprisingly rapid. Carbonate veins in mantle peridotite in Oman have an average 14 C age of ≈26,000 years, and are not 30–95 million years old as previously believed. These data and reconnaissance mapping show that ≈10 4 to 10 5 tons per year of atmospheric CO 2 are converted to solid carbonate minerals via peridotite weathering in Oman. Peridotite carbonation can be accelerated via drilling, hydraulic fracture, input of purified CO 2 at elevated pressure, and, in particular, increased temperature at depth. After an initial heating step, CO 2 pumped at 25 or 30 °C can be heated by exothermic carbonation reactions that sustain high temperature and rapid reaction rates at depth with little expenditure of energy. In situ carbonation of peridotite could consume >1 billion tons of CO 2 per year in Oman alone, affording a low-cost, safe, and permanent method to capture and store atmospheric CO 2 .

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Authors: Kelemen, P. B., & Matter, J.
Affiliations: Lamont-Doherty Earth Observatory (US)
ORCID: Kelemen, Peter B.
Matter, Jürg
Venue: Proceedings of the National Academy of Sciences
Publisher: National Academy of Sciences
Published: 2008-11-11
Volume: 105
Issue: 45
Pages: 17295-17300
ISSN: 0027-8424 (ISSN-L)
1091-6490
DOI: 10.1073/pnas.0805794105
PMC: PMC2582290
OpenAlex: W2102735659
Cited by: 750
References: 39
Citations by year: 2026: 69 · 2025: 71 · 2024: 48 · 2023: 49 · 2022: 46 · 2021: 50 · 2020: 46 · 2019: 30 · 2018: 42 · 2017: 46 · 2016: 32 · 2015: 33 · 2014: 41 · 2013: 47 · 2012: 36
FWCI: 21.96
Type: journal article
Language: en
Open access: green
www.ncbi.nlm.nih.gov
Locations: Proceedings of the National Academy of Sciences (publishedVersion)
PubMed Central (publishedVersion)
ePrints Soton (University of Southampton) (submittedVersion)
Topics: Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Geological and Geochemical Analysis
Keywords: CO2 sequestration, Samail ophiolite, carbonate veins, radiocarbon dating, hydraulic fracturing, Oman

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In situ carbonation of peridotite for CO 2 storage

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