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Cited by 484

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Influence of vapor wall loss in laboratory chambers on yields of secondary organic aerosol

Open access
Zhang, Xuan, Cappa, Christopher D., Jathar, Shantanu H., McVay, Renee C., Ensberg, Joseph J., Kleeman, Michael J., Seinfeld, John H.·2014·Proceedings of the National Academy of Sciences

Abstract

Significance: Atmospheric secondary organic aerosol (SOA) has important impacts on climate and air quality, yet models continue to have difficulty in accurately simulating SOA concentrations. Nearly all SOA models are tied to observations of SOA formation in laboratory chamber experiments. Here, a comprehensive analysis of new experimental results demonstrates that the formation of SOA in laboratory chambers may be substantially suppressed due to losses of SOA-forming vapors to chamber walls, which leads to underestimates of SOA in air-quality and climate models, especially in urban areas where anthropogenic SOA precursors dominate. This analysis provides a time-dependent framework for the interpretation of laboratory chamber experiments that will allow for development of parameterized models of SOA formation that are appropriate for use in atmospheric models.

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Metadata

Authors
Zhang, X., Cappa, C. D., Jathar, S. H., McVay, R. C., Ensberg, J. J., Kleeman, M. J., & Seinfeld, J. H.
Venue
Proceedings of the National Academy of Sciences
Published
2014-04-07
Volume
111
Issue
16
Pages
5802-5807
ISSN
  • 0027-8424 (ISSN-L)
  • 1091-6490
OpenAlex
W1996556904
Cited by
484
References
1
FWCI
32.22
Type
journal article
Language
en
Open access
bronze

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CoChat. (2026). Citation check: Influence of vapor wall loss in laboratory chambers on yields of secondary organic aerosol. https://app.cochat.ai/papers/10.1073/pnas.1404727111
The paper
Zhang, X., Cappa, C. D., Jathar, S. H., McVay, R. C., Ensberg, J. J., Kleeman, M. J., & Seinfeld, J. H. (2014). Influence of vapor wall loss in laboratory chambers on yields of secondary organic aerosol. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.1404727111

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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