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Enhanced strength and temperature dependence of mechanical properties of Li at small scales and its implications for Li metal anodes
Open accessAbstract
Significance: Li metal anodes play a crucial part in next-generation Li ion and “beyond-Li ion” batteries. The issue of dendrites remains a major hurdle, and mechanical suppression through the use of solid electrolytes proves to be a promising solution. However, a lack of knowledge of mechanical properties of lithium metal at the micrometer scale limits our understanding of the mechanical interactions at the electrolyte/electrode interface. In this work, we report results on the mechanical properties of Li, specifically that Li exhibits a strong size effect at room and elevated temperature. First-principle calculations show a high level of elastic anisotropy. Based on the results, we present rational guidelines for anode/electrolyte selection and operating condition that will lead to better cycling performance.
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Special points for Brillouin-zone integrations
Monkhorst, H. J., & Pack, J. D. (1976) · Physical Review B · doi:10.1103/physrevb.13.5188 · Cited by 71,721
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Zhao, Q., Stalin, S., Zhao, C.-Z., & Archer, L. A. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0165-5 · Cited by 2,372
Wang, X., Zeng, W., Hong, L., Xu, W., Yang, H., Wang, F., Duan, H., Tang, M., & Jiang, H. (2018) · Nature Energy · doi:10.1038/s41560-018-0104-5 · Cited by 499
A review of safety-focused mechanical modeling of commercial lithium-ion batteries
Zhu, J., Wierzbicki, T., & Li, W. (2018) · Journal of Power Sources · doi:10.1016/j.jpowsour.2017.12.034 · Cited by 482
Zheng, J., Kim, M. S., Tu, Z., Choudhury, S., Tang, T., & Archer, L. A. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00883g · Cited by 466
Chen, S., Wen, K., Fan, J., Bando, Y., & Golberg, D. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta03358g · Cited by 367
Metadata
- Authors
- Xu, C., Ahmad, Z., Aryanfar, A., Viswanathan, V., & Greer, J. R.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2016-12-19
- Volume
- 114
- Issue
- 1
- Pages
- 57-61
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W2467690158
- Cited by
- 302
- References
- 1
- FWCI
- 7.32
- Type
- journal article
- Language
- en
- Open access
- green
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- Xu, C., Ahmad, Z., Aryanfar, A., Viswanathan, V., & Greer, J. R. (2017). Enhanced strength and temperature dependence of mechanical properties of Li at small scales and its implications for Li metal anodes. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.1615733114
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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