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Ultralow thermal conductivity in all-inorganic halide perovskites
Open accessAbstract
Significance: Discovery of materials with low thermal conductivity in simple, fully dense, and single-crystalline solids has proven extremely challenging. This paper reports the discovery of ultralow thermal conductivity (∼0.4 W⋅m −1 ⋅K −1 ) in single-crystalline, all-inorganic halide perovskite nanowires, which is comparable to their amorphous limit value. We attribute ultralow thermal conductivity to a cluster rattling mechanism, based on strong phonon–phonon scattering via the coexistence of collective motions involving various atom groups. These results call attention to the vital thermal transport processes and thermal management strategies for applications with all-inorganic halide perovskites. Further, CsSnI 3 shows a rare combination of ultralow thermal conductivity and high electrical conductivity, so it can be a promising material for unique applications as an electrically conductive thermal insulator.
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Cites
Thermal properties of graphene and nanostructured carbon materials
Balandin, A. A. (2011) · Nature Materials · doi:10.1038/nmat3064 · Cited by 6,244
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
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Anharmoncity and low thermal conductivity in thermoelectrics
Chang, C., & Zhao, L.-D. (2018) · Materials Today Physics · doi:10.1016/j.mtphys.2018.02.005 · Cited by 359
Robot-Accelerated Perovskite Investigation and Discovery
Li, Z., Najeeb, M. A., Alves, L., Sherman, A. Z., Shekar, V., Cruz Parrilla, P., Pendleton, I. M., Wang, W., Nega, P. W., Zeller, M., et al. (2020) · Chemistry of Materials · doi:10.1021/acs.chemmater.0c01153 · Cited by 187
High-bandwidth perovskite photonic sources on silicon
Ren, A., Wang, H., Dai, L., Xia, J., Bai, X., Butler-Caddle, E., Smith, J. A., Lai, H., Ye, J., Li, X., et al. (2023) · Nature Photonics · doi:10.1038/s41566-023-01242-9 · Cited by 49
Advances in femtosecond laser synthesis and micromachining of halide perovskites
Du, S., Zhang, F., & Ma, L. (2024) · Light: Advanced Manufacturing · doi:10.37188/lam.2024.035 · Cited by 9
Thermal conductivity of polar nitride perovskite LaWN3
Liu, Y., Zhou, X., Wang, S., & Sun, B. (2025) · Modern Physics Letters B · doi:10.1142/s0217984925500526 · Cited by 3
Metadata
- Authors
- Lee, W., Li, H., Wong, A. B., Zhang, D., Lai, M., Yu, Y., Kong, Q., Lin, E., Urban, J. J., Grossman, J. C., & Yang, P.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2017-07-31
- Volume
- 114
- Issue
- 33
- Pages
- 8693-8697
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W2740039296
- Cited by
- 412
- References
- 5
- FWCI
- 10.84
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Lee, W., Li, H., Wong, A. B., Zhang, D., Lai, M., Yu, Y., Kong, Q., Lin, E., Urban, J. J., Grossman, J. C., & Yang, P. (2017). Ultralow thermal conductivity in all-inorganic halide perovskites. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.1711744114
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