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Thermal non-equilibrium transport in colloids
Open accessAbstract
A temperature gradient acts like an external field on colloidal suspensions and drives the solute particles to the cold or to the warm, depending on interfacial and solvent properties. We discuss different transport mechanisms for charged colloids, and how a thermal gradient gives rise to companion fields. Particular emphasis is put on the thermal response of the electrolyte solution: positive and negative ions diffuse along the temperature gradient and thus induce a thermoelectric field which in turn acts on the colloidal charges. Regarding polymers in organic solvents, the physical mechanism changes with decreasing molecular weight: high polymers are described in the framework of macroscopic hydrodynamics; for short chains and molecular mixtures of similar size, the Brownian motion of solute and solvent becomes important.
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Cites
Extreme accumulation of nucleotides in simulated hydrothermal pore systems
Baaske, P., Weinert, F. M., Duhr, S., Lemke, K. H., Russell, M. J., & Braun, D. (2007) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0609592104 · Cited by 367
Formation of Protocell-like Vesicles in a Thermal Diffusion Column
Budin, I., Bruckner, R. J., & Szostak, J. W. (2009) · Journal of the American Chemical Society · doi:10.1021/ja9029818 · Cited by 132
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Osmosis, from molecular insights to large-scale applications
Marbach, S., & Bocquet, L. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00420j · Cited by 316
Accumulation of formamide in hydrothermal pores to form prebiotic nucleobases
Niether, D., Afanasenkau, D., Dhont, J. K. G., & Wiegand, S. (2016) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.1600275113 · Cited by 88
Steady Out‐of‐Equilibrium Chemistry: What? Why? How?
Plasson, R., & Jullien, L. (2025) · ChemSystemsChem · doi:10.1002/syst.202500011 · Cited by 3
Metadata
- Authors
- Würger, A.
- Venue
- Reports on Progress in Physics
- Publisher
- IOP Publishing
- Published
- 2010-11-18
- Volume
- 73
- Issue
- 12
- Pages
- 126601
- ISSN
- 0034-4885 (ISSN-L)
- 1361-6633
- OpenAlex
- W2044699539
- Cited by
- 433
- References
- 2
- FWCI
- 9.55
- Type
- journal article
- Language
- en
- Open access
- bronze
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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