Cited by 351Carbon Dioxide Capture TechnologiesZeolite Catalysis and SynthesisCO2 Sequestration and Geologic Interactions

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Advances in principal factors influencing carbon dioxide adsorption on zeolites

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Bonenfant, Danielle, Kharoune, Mourad, Niquette, Patrick, Mimeault, Murielle, Hausler, Robert·2008·Science and Technology of Advanced Materials

DOI 10.1088/1468-6996/9/1/013007PMC PMC5099794

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Abstract

We report the advances in the principal structural and experimental factors that might influence the carbon dioxide (CO2) adsorption on natural and synthetic zeolites. The CO2 adsorption is principally govern by the inclusion of exchangeable cations (countercations) within the cavities of zeolites, which induce basicity and an electric field, two key parameters for CO2 adsorption. More specifically, these two parameters vary with diverse factors including the nature, distribution and number of exchangeable cations. The structure of framework also determines CO2 adsorption on zeolites by influencing the basicity and electric field in their cavities. In fact, the basicity and electric field usually vary inversely with the Si/Al ratio. Furthermore, the CO2 adsorption might be limited by the size of pores within zeolites and by the carbonates formation during the CO2 chemisorption. The polarity of molecules adsorbed on zeolites represents a very important factor that influences their interaction with the electric field. The adsorbates that have the most great quadrupole moment such as the CO2, might interact strongly with the electric field of zeolites and this favors their adsorption. The pressure, temperature and presence of water seem to be the most important experimental conditions that influence the adsorption of CO2. The CO2 adsorption increases with the gas phase pressure and decreases with the rise of temperature. The presence of water significantly decreases adsorption capacity of cationic zeolites by decreasing strength and heterogeneity of the electric field and by favoring the formation of bicarbonates. The optimization of the zeolites structural characteristics and the experimental conditions might enhance substantially their CO2 adsorption capacity and thereby might give rise to the excellent adsorbents that may be used to capturing the industrial emissions of CO2.

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Authors: Bonenfant, D., Kharoune, M., Niquette, P., Mimeault, M., & Hausler, R.
Affiliations: École de Technologie Supérieure (CA)
University of Nebraska Medical Center (US)
STEPPE-École de Technologie Supérieure, Département de Génie de la Construction, 1100, Notre-Dame Ouest, Montréal, QC, H3C 1K3, Canada
Venue: Science and Technology of Advanced Materials
Publisher: Informa UK Limited
Published: 2008-01
Volume: 9
Issue: 1
Pages: 013007
ISSN: 1468-6996 (ISSN-L)
1878-5514
DOI: 10.1088/1468-6996/9/1/013007
PMC: PMC5099794
OpenAlex: W2114992971
Cited by: 351
References: 67
Citations by year: 2026: 26 · 2025: 37 · 2024: 25 · 2023: 31 · 2022: 26 · 2021: 25 · 2020: 17 · 2019: 24 · 2018: 16 · 2017: 17 · 2016: 16 · 2015: 17 · 2014: 15 · 2013: 15 · 2012: 16
FWCI: 19.82
Type: journal article
Language: en
Open access: gold
doi.org
Locations: Science and Technology of Advanced Materials (publishedVersion)
PubMed Central (publishedVersion)
PubMed (publishedVersion)
Funders: Natural Sciences and Engineering Research Council of Canada
Topics: Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Physical Sciences › Chemistry › Inorganic Chemistry › Zeolite Catalysis and Synthesis
Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
Keywords: CO2 adsorption, zeolites, exchangeable cations, zeolite basicity, electric field, Si/Al ratio, framework structure, pore size, carbonate formation, CO2 chemisorption, water effect, temperature and pressure dependence, CO2 capture, industrial emissions

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Advances in principal factors influencing carbon dioxide adsorption on zeolites

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