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Cited by 25Hydrogels: synthesis, properties, applicationsAdsorption and biosorption for pollutant removalAdvanced Cellulose Research Studies

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Enhancement of mechanical property and absorption capability of hydrophobically associated polyacrylamide hydrogels by adding cellulose nanofiber

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Zhang, Yiyin, Zhao, Xueyang, Yang, Weixing, Jiang, Weijiao, Chen, Feng, Fu, Qiang·2020·Materials Research Express
DOI 10.1088/2053-1591/ab6373
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Abstract

Hydrophobically associated (HA) hydrogels have attracted great concerns with their admirable properties, such as self-healing and shape memory. However, a few works have been devoted to apply HA hydrogels in practice, especially in wastewater treatment. This may be because of the non-ionic monomer composition and the poor mechanical properties after swelling. In this work, in order to improve the mechanical properties and absorption behavior of HA polyacrylamide (HPAM) hydrogel, hydrophobically associated polyacrylamide/cellulose nanofiber (HPAMF) composite hydrogels were prepared. It was found that by incorporating CNF (2 wt%), the tensile strength (≈0.276 MPa) was largely increased by 632% compared to HPAM hydrogels. The maximum Cu ion adsorption capacity of the HPAMF hydrogel (containing 2 wt% CNF) was 2.33 mmol g−1, about 86% over the HPAM hydrogel. The HPAMF hydrogels with self-healing, excellent mechanical and adsorption properties can be promisingly served as reliable absorbents, consequently satisfying the needs of practical application of heavy metal treatment.

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Research works printed but not linked: 52

  1. Strassburg, 2017, Cross-linking of a hydrophilic, antimicrobial polycation toward a fast-swelling, antimicrobial superabsorber and interpenetrating hydrogel networks with long lasting antimicrobial properties, ACS Applied Materials & Interfaces, 9, 36573, 10.1021/acsami.7b10049 · DOI
  2. Sekine, 2014, Dependence of structure of polymer side chain on water structure in hydrogels, Polymer, 55, 6320, 10.1016/j.polymer.2014.10.011 · DOI
  3. Alam, 2016, Electrically conductive, mechanically robust, pH-sensitive graphene/polymer composite hydrogels, Compos. Sci. Technol., 127, 119, 10.1016/j.compscitech.2016.02.024 · DOI
  4. Duan, 2017, Robust and smart hydrogels based on natural polymers, Chin. J. Polym. Sci., 35, 1165, 10.1007/s10118-017-1983-9 · DOI
  5. Cao, 2018, Controlled cross-linking strategy for formation of hydrogels, microgels and nanogels, Chin. J. Polym. Sci., 36, 8, 10.1007/s10118-018-2061-7 · DOI
  6. Ge, 2018, Stretchable, transparent, and self-patterned hydrogel-based pressure sensor for human motions detection, Adv. Funct. Mater., 28, 10.1002/adfm.201802576 · DOI · Paper page
  7. Yang, 2018, Robust and mechanically and electrically self-healing hydrogel for efficient electromagnetic interference shielding, ACS Applied Materials & Interfaces, 10, 8245, 10.1021/acsami.7b18700 · DOI
  8. Cho, 2018, Ascidian-inspired fast-forming hydrogel system for versatile biomedical applications: pyrogallol chemistry for dual modes of crosslinking mechanism, Adv. Funct. Mater., 28, 10.1002/adfm.201705244 · DOI
  9. Li, 2019, Highly stretchable ionic conducting hydrogels for strain/tactile sensors, Polymer, 167, 154, 10.1016/j.polymer.2019.01.038 · DOI
  10. Tang, 2019, Design of low temperature-responsive hydrogels used as a temperature indicator, Polymer, 173, 182, 10.1016/j.polymer.2019.04.052 · DOI
  11. Li, 2018, Hierarchically crosslinked ionic nanocomposite hydrogels with ultrahigh mechanical properties for underwater bioinspired capturing device, Compos. Sci. Technol., 165, 339, 10.1016/j.compscitech.2018.07.018 · DOI
  12. Zeng, 2014, Preparation and characterization of Poly(γ-glutamic acid) hydrogels as potential tissue engineering scaffolds, Chin. J. Polym. Sci., 32, 1507, 10.1007/s10118-014-1536-4 · DOI
  13. Wang, 2020, Rhodamine mechanophore functionalized mechanochromic double network hydrogels with high sensitivity to stress, Chin. J. Polym. Sci, 38, 24, 10.1007/s10118-019-2293-1 · DOI
  14. Zhang, 2018, Tough poly(L-DOPA)-containing double network hydrogel beads with high capacity of dye adsorption, Chin. J. Polym. Sci., 36, 1251, 10.1007/s10118-018-2163-2 · DOI
  15. Brown, 2007, A model of the fracture of double network gels, Macromolecules, 40, 3815, 10.1021/ma062642y · DOI
  16. Mora, 2011, The kinetic approach to fracture in transient networks, Soft Matter, 7, 4908, 10.1039/c0sm01203c · DOI
  17. Sun, 2019, Self-healing hydrogels with stimuli responsiveness based on acylhydrazone bonds, Polymer, 160, 246, 10.1016/j.polymer.2018.11.051 · DOI
  18. Yang, 2014, Keys to enhancing mechanical properties of silica nanoparticle composites hydrogels: the role of network structure and interfacial interactions, Compos. Sci. Technol., 95, 1, 10.1016/j.compscitech.2014.02.003 · DOI
  19. Jiang, 2010, Network structure and compositional effects on tensile mechanical properties of hydrophobic association hydrogels with high mechanical strength, Polymer, 51, 1507, 10.1016/j.polymer.2010.01.061 · DOI
  20. Abdurrahmanoglu, 2009, Design of high-toughness polyacrylamide hydrogels by hydrophobic modification, Polymer, 50, 5449, 10.1016/j.polymer.2009.09.042 · DOI
  21. Tuncaboylu, 2011, Tough and self-healing hydrogels formed via hydrophobic interactions, Macromolecules, 44, 4997, 10.1021/ma200579v · DOI
  22. Owusu-Nkwantabisah, 2018, Thermal stiffening of hydrophobic association hydrogels, Polymer, 145, 374, 10.1016/j.polymer.2018.05.022 · DOI
  23. Cui, 2015, Robust, anti-fatigue, and self-healing graphene oxide/hydrophobically associated composite hydrogels and their use as recyclable adsorbents for dye wastewater treatment, Journal of Materials Chemistry A, 3, 17445, 10.1039/C5TA04470G · DOI
  24. Liu, 2018, A simple coordination strategy for preparing a complex hydrophobic association hydrogel, J. Appl. Polym. Sci., 135, 46400, 10.1002/app.46400 · DOI
  25. Imato, 2012, Self-healing of chemical gels cross-linked by diarylbibenzofuranone-based trigger-free dynamic covalent bonds at room temperature, Angew. Chem. Int. Ed., 51, 1138, 10.1002/anie.201104069 · DOI
  26. Burattini, 2009, A self-repairing, supramolecular polymer system: healability as a consequence of donor–acceptor π–π stacking interactions, Chem. Commun., 6717, 10.1039/b910648k · DOI
  27. Chen, 2012, Multiphase design of autonomic self-healing thermoplastic elastomers, Nat. Chem., 4, 467, 10.1038/nchem.1314 · DOI
  28. Nakahata, 2011, Redox-responsive self-healing materials formed from host–guest polymers, Nat. Commun., 2, 511, 10.1038/ncomms1521 · DOI
  29. Cui, 2015, Robust dual physically cross-linked hydrogels with unique self-reinforcing behavior and improved dye adsorption capacity, RSC Adv., 5, 52966, 10.1039/C5RA06361B · DOI
  30. Saito, 2007, Cellulose nanofibers prepared by TEMPO-mediated oxidation of native cellulose, Biomacromolecules, 8, 2485, 10.1021/bm0703970 · DOI · Paper page
  31. Isogai, 2011, TEMPO-oxidized cellulose nanofibers, Nanoscale, 3, 71, 10.1039/C0NR00583E · DOI
  32. Yang, 2017, Completely green approach for the preparation of strong and highly conductive graphene composite film by using nanocellulose as dispersing agent and mechanical compression, ACS Sustainable Chemistry & Engineering, 5, 9102, 10.1021/acssuschemeng.7b02012 · DOI
  33. Xu, 2018, Electric field-induced alignment of nanofibrillated cellulose in thermoplastic polyurethane matrix, Compos. Sci. Technol., 156, 117, 10.1016/j.compscitech.2017.12.017 · DOI
  34. Xu, 2017, Largely enhanced stretching sensitivity of polyurethane/carbon nanotube nanocomposites via incorporation of cellulose nanofiber, The Journal of Physical Chemistry C, 121, 2108, 10.1021/acs.jpcc.6b11783 · DOI
  35. Wu, 2018, Preparation of a thermally conductive biodegradable cellulose nanofiber/hydroxylated boron nitride nanosheet film: the critical role of edge-hydroxylation, Journal of Materials Chemistry A, 6, 11863, 10.1039/C8TA03642J · DOI
  36. Shinoda, 2012, Relationship between length and degree of polymerization of TEMPO-oxidized cellulose nanofibrils, Biomacromolecules, 13, 842, 10.1021/bm2017542 · DOI
  37. Zhu, 2019, Highly sensitive, ultrastretchable strain sensors prepared by pumping hybrid fillers of carbon nanotubes/cellulose nanocrystal into electrospun polyurethane membranes, ACS Applied Materials & Interfaces, 11, 12968, 10.1021/acsami.9b00136 · DOI
  38. Qiu, 2018, Super strong all-cellulose composite filaments by combination of inducing nanofiber formation and adding nanofibrillated cellulose, Biomacromolecules, 19, 4386, 10.1021/acs.biomac.8b01262 · DOI
  39. Chen, 2018, Highly conductive nanocomposites based on cellulose nanofiber networks via NaOH treatments, Compos. Sci. Technol., 156, 103, 10.1016/j.compscitech.2017.12.029 · DOI
  40. Shakeri, 2011, Water repellent cellulose nanofibers by acetylation, Advanced Materials Research, 332-334, 209, 10.4028/www.scientific.net/AMR.332-334.209 · DOI
  41. Ashori, 2014, Solvent-free acetylation of cellulose nanofibers for improving compatibility and dispersion, Carbohydrate Polym., 102, 369, 10.1016/j.carbpol.2013.11.067 · DOI
  42. Niu, 2018, Dual physically crosslinked healable polyacrylamide/cellulose nanofibers nanocomposite hydrogels with excellent mechanical properties, Carbohydrate Polym., 193, 73, 10.1016/j.carbpol.2018.03.086 · DOI
  43. Du, 2019, Cellulose nanocrystals and cellulose nanofibrils based hydrogels for biomedical applications, Carbohydrate Polym., 209, 130, 10.1016/j.carbpol.2019.01.020 · DOI
  44. Chen, 2017, Facile approach to the fabrication of 3D cellulose nanofibrils (CNFs) reinforced poly(vinyl alcohol) hydrogel with ideal biocompatibility, Carbohydrate Polym., 173, 547, 10.1016/j.carbpol.2017.06.036 · DOI
  45. Yin, 2017, Improvement in mechanical properties and biocompatibility of biosynthetic bacterial cellulose/lotus root starch composites, Chin. J. Polym. Sci., 35, 354, 10.1007/s10118-017-1903-z · DOI
  46. Siró, 2010, Microfibrillated cellulose and new nanocomposite materials: a review, Cellulose, 17, 459, 10.1007/s10570-010-9405-y · DOI
  47. Jiang, 2019, Hydrophobic association hydrogels with excellent mechanical and self-healing properties, Eur. Polym. J, 112, 660, 10.1016/j.eurpolymj.2018.10.031 · DOI
  48. Yang, 2010, Temperature-responsive properties of poly(acrylic acid-co-acrylamide) hydrophobic association hydrogels with high mechanical strength, Macromolecules, 43, 10645, 10.1021/ma1022555 · DOI
  49. Tang, 2012, Adsorption isotherms and kinetics studies of malachite green on chitin hydrogels, J. Hazard. Mater., 209-210, 218, 10.1016/j.jhazmat.2012.01.010 · DOI
  50. Zheng, 2010, Adsorption behavior of Cu2+ from aqueous solutions onto starch-g-poly(acrylic acid)/sodium humate hydrogels, Desalination, 263, 170, 10.1016/j.desal.2010.06.054 · DOI
  51. Mallakpour, 2019, Poly(vinyl alcohol)/Vitamin C-multi walled carbon nanotubes composites and their applications for removal of methylene blue: Advanced comparison between linear and nonlinear forms of adsorption isotherms and kinetics models, Polymer, 160, 115, 10.1016/j.polymer.2018.11.035 · DOI
  52. Isobe, 2013, TEMPO-oxidized cellulose hydrogel as a high-capacity and reusable heavy metal ion adsorbent, J. Hazard. Mater., 260, 195, 10.1016/j.jhazmat.2013.05.024 · DOI

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Metadata

Authors
Zhang, Y., Zhao, X., Yang, W., Jiang, W., Chen, F., & Fu, Q.
Affiliations
Sichuan University (CN)
Corresponding author
  • Chen, Feng
  • Fu, Qiang
ORCID
Venue
Materials Research Express
Publisher
IOP Publishing
Published
2020-01-01
Volume
7
Issue
1
Pages
015319
ISSN
2053-1591 (ISSN-L)
DOI
10.1088/2053-1591/ab6373
OpenAlex
W2994650056
Cited by
25
References
0
Citations by year
2026: 1 · 2025: 4 · 2024: 5 · 2023: 5 · 2022: 3 · 2021: 4 · 2020: 3
FWCI
0.86
Type
journal article
Language
en
Open access
Licence
Locations
  • Materials Research Express (publishedVersion, cc-by)
  • DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion)
Funders
National Natural Science Foundation of China (Grant No. 51721091 and 51573102)
Topics
  • Physical Sciences › Materials Science › Biomaterials › Hydrogels: synthesis, properties, applications
  • Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
  • Physical Sciences › Materials Science › Biomaterials › Advanced Cellulose Research Studies
Keywords
polyacrylamide hydrogel, cellulose nanofibers, composite hydrogels, tensile strength, heavy metal adsorption, copper adsorption, self-healing hydrogels, wastewater treatment, absorbing materials

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