The DOI matches its Crossref record; 65 of the 65 references it cites were found in a registry or an index.
Organic light-emitting diodes: theoretical understanding of highly efficient materials and development of computational methodology
Open accessAbstract
Theoretical understanding of organic light-emitting diodes started from the quest to the nature of the primary excitation in organic molecular and polymeric materials. We found the electron correlation strength, bond-length alternation as well as the conjugation extent have strong influences on the orderings of the lowest lying excited states through the first application of density matrix renormalization group theory to quantum chemistry. The electro-injected free carriers (with spin 1/2) can form both singlet and triplet bound states. We found that the singlet exciton formation ratio can exceed the conventional 25% spin statistics limit. We proposed a vibration correlation function formalism to evaluate the excited-state decay rates, which is shown to not only give reasonable estimations for the quantum efficiency but also a quantitative account for the aggregation-induced emission (AIE). It is suggested to unravel the AIE mechanism through resonance Raman spectroscopy.
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Cites
Organic electroluminescent diodes
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Light-emitting diodes based on conjugated polymers
Burroughes, J. H., Bradley, D. D. C., Brown, A. R., Marks, R. N., Mackay, K., Friend, R. H., Burns, P. L., & Holmes, A. B. (1990) · Nature · doi:10.1038/347539a0 · Cited by 11,393
Aggregation-induced emission of 1-methyl-1,2,3,4,5-pentaphenylsilole
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Aggregation-Induced Emission: Together We Shine, United We Soar!
Mei, J., Leung, N. L. C., Kwok, R. T. K., Lam, J. W. Y., & Tang, B. Z. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00263 · Cited by 8,270
Highly efficient organic light-emitting diodes from delayed fluorescence
Uoyama, H., Goushi, K., Shizu, K., Nomura, H., & Adachi, C. (2012) · Nature · doi:10.1038/nature11687 · Cited by 8,188
Highly efficient phosphorescent emission from organic electroluminescent devices
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Nearly 100% internal phosphorescence efficiency in an organic light-emitting device
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Aggregation‐Induced Emission: The Whole Is More Brilliant than the Parts
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Cited by
Ma, H., Peng, Q., An, Z., Huang, W., & Shuai, Z. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.8b11224 · Cited by 613
Self-citationConstitutional Isomerization Enables Bright NIR‐II AIEgen for Brain‐Inflammation Imaging
Liu, S., Chen, C., Li, Y., Zhang, H., Liu, J., Wang, R., Wong, S. T. H., Lam, J. W. Y., Ding, D., & Tang, B. Z. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201908125 · Cited by 267
Tu, Y., Liu, J., Zhang, H., Peng, Q., Lam, J. W. Y., & Tang, B. Z. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201907522 · Cited by 180
Self-citation
Metadata
- Authors
- Shuai, Z., & Peng, Q.
- Venue
- National Science Review
- Publisher
- Oxford University Press (OUP)
- Published
- 2016-04-19
- Volume
- 4
- Issue
- 2
- Pages
- 224-239
- ISSN
- 2053-714X (ISSN-L)
- 2095-5138
- OpenAlex
- W2341273646
- Cited by
- 375
- References
- 65
- FWCI
- 5.79
- Type
- journal article
- Language
- en
- Open access
- hybrid
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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