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Cited by 275

The DOI matches its Crossref record; 26 of the 26 references it cites were found in a registry or an index.

Optical studies of the a-,b-, and c-axis charge dynamics inYBa2Cu3O6+x

Cooper, S. L., Reznik, D., Kotz, A., Karlow, M. A., Liu, R., Klein, M. V., Lee, W. C., Giapintzakis, J., Ginsberg, D. M., Veal, B. W., Paulikas, A. P.·1993·Physical Review B

Abstract

Optical and Raman-scattering studies of a-, b-, and c-axis ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$ between 0.025 and 5.5 eV are presented as a function of doping, and compared to the results of ${\mathrm{Bi}}_{2}$${\mathrm{Sr}}_{2}$${\mathrm{CaCu}}_{2}$${\mathrm{O}}_{8}$ and ${\mathrm{La}}_{2\mathrm{\ensuremath{-}}\mathit{x}}$${\mathrm{Sr}}_{\mathit{x}}$${\mathrm{CuO}}_{4}$. Our doping-dependence studies show that the redistribution of spectral weight in the ${\mathrm{CuO}}_{2}$ planes of ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$ differs significantly from that seen in ${\mathrm{La}}_{2\mathrm{\ensuremath{-}}\mathit{x}}$${\mathrm{Sr}}_{\mathit{x}}$${\mathrm{CuO}}_{4}$. We also find that the redistribution of spectral weight in the cuprates is primarily responsible for the loss of two-magnon Raman-scattering intensity with doping. Finally, we show that bound-carrier contributions comprise a significantly larger fraction of the spectral weight below 1 eV in lower-${\mathit{T}}_{\mathit{c}}$ cuprates such as the 2:1:4 compounds than in higher-${\mathit{T}}_{\mathit{c}}$ cuprates such as ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$ and ${\mathrm{Bi}}_{2}$${\mathrm{Sr}}_{2}$${\mathrm{CaCu}}_{2}$${\mathrm{O}}_{8}$.We suggest that the low-frequency conductivity (1 eV) in the 2:1:4 compounds is most appropriately described by a two-component picture, while that in ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$ and ${\mathrm{Bi}}_{2}$${\mathrm{Sr}}_{2}$${\mathrm{CaCu}}_{2}$${\mathrm{O}}_{8}$ is adequately described as a single component of strongly interacting carriers. In the metallic phase we find several interesting consequences of a single-component interpretation of the optical data in ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$, such as a linear-in-\ensuremath{\omega} frequency-dependent scattering rate and an increase in the interaction strength with decreased carrier density. Finally, we show that the c-axis optical response in ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{7}$ (${\mathit{T}}_{\mathit{c}}$\ensuremath{\sim}90 K) is characterized by a c-axis polarized Raman continuum and a Drude conductivity arising from interbilayer charge transport along the c direction. With decreased doping, the c-axis Drude response decreases dramatically, indicating a decoupling of the ${\mathrm{CuO}}_{2}$ plane bilayers in ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$. By comparison, the ab-plane optical response is not strongly influenced by interbilayer decoupling, suggesting that the unusual ab-plane charge dynamics in ${\mathrm{YBa}}_{2}$${\mathrm{Cu}}_{3}$${\mathrm{O}}_{6+\mathit{x}}$ persist in nearly isolated ${\mathrm{CuO}}_{2}$ plane bilayers.

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Crossref · 10.1103/physrevb.47.8233

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Metadata

Authors
Cooper, S. L., Reznik, D., Kotz, A., Karlow, M. A., Liu, R., Klein, M. V., Lee, W. C., Giapintzakis, J., Ginsberg, D. M., Veal, B. W., & Paulikas, A. P.
Venue
Physical Review B
Published
1993-04-01
Volume
47
Issue
13
Pages
8233-8248
ISSN
  • 0163-1829 (ISSN-L)
  • 1095-3795
OpenAlex
W2007695511
Cited by
275
References
26
FWCI
16.96
Type
journal article
Language
en
Open access
closed

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