Rare-Gas Clusters in Intense Extreme-Ultraviolet Pulses from a High-Order Harmonic Source
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We report evidence for two previously unidentified effects in the ionization of rare-gas clusters by intense extreme-ultraviolet pulses. First, electron spectra indicate multistep photoemission with increasing isotropy for larger clusters due to electron-atom collisions. Second, very slow (meV) electrons are interpreted as the first experimental evidence for Rydberg-like atomic state formation in the nanoplasma expansion. Only small fractions of Xe2+ ions were found, in sharp contrast to previous results recorded under comparable conditions [Murphy et al., Phys. Rev. Lett. 101, 203401 (2008).
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We have measured ionization and recombination dynamics in large rare-gas clusters and observed XUV-induced Rabi oscillations in two-color double ionization of Ar.
“As an example of (1), we have measured ionization and recombination dynamics in large rare-gas clusters [182,183] and have observed XUV-induced Rabi oscillations in two-color double ionization of Ar [184]”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [183]
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Ionization dynamics of Xe nanoplasma formation studied with XUV fluorescence spectroscopy
Przystawik, A., Schroedter, L., Müller, M., Adolph, M., Bostedt, C., Flückiger, L., Gorkhover, T., Kickermann, A., Krikunova, M., Nösel, L., et al. (2015) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/48/18/184002 · Cited by 3 · see citing works
Tracing transient charges in expanding clusters
Schütte, B., Vrakking, M. J. J., & Rouzée, A. (2017) · Physical Review A · doi:10.1103/physreva.95.063417 · Cited by 4 · see citing works
Self-citationSlow electrons from clusters in strong x-ray pulses
Garibay, A. C., Saalmann, U., & Rost, J. M. (2015) · Journal of Physics B Atomic Molecular and Optical Physics · doi:10.1088/0953-4075/48/17/174003 · Cited by 3 · see citing works
Slow electrons from clusters in strong x-ray pulses
Garibay, A. C., Saalmann, U., & Rost, J. M. (2015) · MPG.PuRe (Max Planck Society) · Cited by 3 · see citing works
Time Evolution of Coulomb Explosion of Argon Clusters in Moderately Intense Nanosecond Laser Fields
Tran, K. C., Tran, S., Rios, G., & Kong, W. (2025) · The Journal of Physical Chemistry A · doi:10.1021/acs.jpca.5c07047 · Cited by 2 · see citing works
Klimešová, E., Kulyk, O., Martin, L. J., Schütte, B., Frühling, U., Drescher, M., Pan, R., Stojanovic, N., Macias, I. J. B., Düsterer, S., et al. (2025) · New Journal of Physics · doi:10.1088/1367-2630/ada575 · Cited by 2 · see citing works
Self-citationCorrelated electronic decay following intense near-infrared ionization of clusters
Schütte, B., Arbeiter, M., Fennel, T., Jabbari, G., Kuleff, A. I., Vrakking, M. J. J., & Rouzée, A. (2015) · Journal of Physics Conference Series · doi:10.1088/1742-6596/635/1/012025 · Cited by 2 · see citing works
Self-citationMultispectroscopic Study of Single Xe Clusters Using XFEL Pulses
Nishiyama, T., Bostedt, C., Ferguson, K., Hutchison, C. D. M., Nagaya, K., Fukuzawa, H., Motomura, K., Wada, S., Sakai, T., Matsunami, K., et al. (2019) · Applied Sciences · doi:10.3390/app9224932 · Cited by 2 · see citing works
Imaging Clusters and Their Dynamics with Single-shot Coherent Diffraction
Colombo, A., & Rupp, D. (2023) · Royal Society of Chemistry eBooks · doi:10.1039/bk9781837671564-00172 · Cited by 1 · see citing works
Tracing Nonlinear Cluster Dynamics Induced by Intense XUV, NIR and MIR Laser Pulses
Schütte, B. (2017) · Springer series in chemical physics · doi:10.1007/978-3-319-64840-8_5 · Cited by 1 · see citing works
Self-citationRecombination-Induced Autoionization Process in Rare-Gas Clusters
Schütte, B., Arbeiter, M., Fennel, T., Campi, F., Vrakking, M. J. J., & Rouzée, A. (2015) · Springer proceedings in physics · doi:10.1007/978-3-319-13242-6_14
Self-citationMid-infrared strong-field ionization of clusters using two-cycle pulsesPreprint
Schütte, B., Ye, P., Patchkovskii, S., Austin, D. R., Brahms, C., Strüber, C., Witting, T., Ivanov, M., Tisch, J. W. G., & Marangos, J. P. (2016) · arXiv (Cornell University)
Self-citationIntracluster Coulombic decay following intense NIR ionization of clusters
Schütte, B., Arbeiter, M., Fennel, T., Jabbari, G., Gokhberg, K., Kuleff, A. I., Vrakking, M. J. J., & Rouzée, A. (2015) · Journal of Physics Conference Series · doi:10.1088/1742-6596/635/10/102004
Self-citationTime-resolved investigation of transient charges in laser-produced nanoplasmas
Schütte, B., Vrakking, M. J. J., & Rouzée, A. (2015) · Journal of Physics Conference Series · doi:10.1088/1742-6596/635/10/102005
Self-citationNIR ionization avalanching in clusters ignited by ultrashort XUV pulses
Schütte, B., Arbeiter, M., Mermillod‐Blondin, A., Vrakking, M. J. J., Rouzée, A., & Fennel, T. (2016) · International Conference on Ultrafast Phenomena · doi:10.1364/up.2016.uth4a.40
Self-citationContinuously tunable UV-driven high-intensity HHG source for user applications
Jurkovič, M., Hort, O., Finke, O., Albrecht, M., Roos, A. H., Hoque, Z., Shaw, K., Klimešová, E., Ltaief, L. B., Andreasson, J., et al. (2022) · International Conference on Ultrafast Phenomena · doi:10.1364/up.2022.th4a.23
Ionization of Xenon Clusters by a Hard X-ray Laser Pulse
Kumagai, Y., Xu, W., Asa, K., Nishiyama, T., Motomura, K., Wada, S., Iablonskyi, D., Mondal, S., Tachibana, T., Ito, Y., et al. (2023) · Applied Sciences · doi:10.3390/app13042176
Electron thermalization in ammonia clusters induced by femtosecond laser fields
Yang, T., Zhang, D., Zhao, H., Li, W., Wei, M., Ma, P., He, L., & Ding, D. (2025) · Chemical Physics Letters · doi:10.1016/j.cplett.2025.142074
- Authors
- Schütte, B., Arbeiter, M., Fennel, T., Vrakking, M. J. J., & Rouzée, A.
- Affiliations
- Max-Born-Institute for Nonlinear Optics and Short Pulse Spectroscopy (DE)
- University of Rostock (DE)
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2014-02-20
- Volume
- 112
- Issue
- 7
- Pages
- 073003-073003
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2016622499
- Cited by
- 63
- References
- 35
- Citations by year
- 2025: 3 · 2024: 2 · 2023: 3 · 2022: 1 · 2021: 4 · 2020: 8 · 2019: 3 · 2018: 5 · 2017: 7 · 2016: 11 · 2015: 14 · 2014: 2
- FWCI
- 5.64
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- Refubium (Universitätsbibliothek der Freien Universität Berlin) (submittedVersion)
- Universitätsbibliothek der FU Berlin Hochschulschriftenstelle u. Dokumentenserver
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Nuclear and High Energy Physics › Laser-Plasma Interactions and Diagnostics
- Keywords
- rare gas clusters, extreme ultraviolet pulses, high harmonic generation, cluster ionization, electron-atom collisions, electron spectra, low-energy electrons
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